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Record W2108973738 · doi:10.1002/047084289x.rd382

Dimethyl Sulfoxide-Sulfur Trioxide/Pyridine

2001· reference-entry· en· W2108973738 on OpenAlexaff
Thomas T. Tidwell

Bibliographic record

VenueEncyclopedia of Reagents for Organic Synthesis · 2001
Typereference-entry
Languageen
FieldBiochemistry, Genetics and Molecular Biology
TopicChemical Synthesis and Analysis
Canadian institutionsUniversity of Toronto
Fundersnot available
KeywordsPyridineChemistryReagentSulfur trioxideThionyl chlorideDimethyl sulfoxideSolubilityMedicinal chemistrySulfurOrganic chemistryNuclear chemistrySulfuric acidChloride

Abstract

fetched live from OpenAlex

(DMSO) [67-68-5] C2H6OS (MW 78.13) InChI = 1S/C2H6OS/c1-4(2)3/h1-2H3 InChIKey = IAZDPXIOMUYVGZ-UHFFFAOYSA-N (SO3) [7446-11-9] O3S (MW 80.06) InChI = 1S/O3S/c1-4(2)3 InChIKey = AKEJUJNQAAGONA-UHFFFAOYSA-N (SO3/pyridine) [26412-87-3] C5H5NO3S (MW 159.16) InChI = 1S/C5H5N.O3S/c1-2-4-6-5-3-1;1-4(2)3/h1-5H; InChIKey = UDYFLDICVHJSOY-UHFFFAOYSA-N (oxidant for the conversion of primary and secondary alcohols to aldehydes and ketones, respectively; avoids overoxidation to carboxylic acids; gives very good yields with short reaction times near rt with minimal formation of byproducts) Alternate Name: Parikh–Doering reagent. Physical Data: DMSO: mp 18.4 °C; bp 189 °C; d 1.101 g cm−3. SO3: mp 16.8 °C; bp 44.7 °C; d 1.970 g cm−3. SO3/pyridine: mp 175 °C. Solubility: DMSO: sol H2O, alcohol, acetone, THF, CH2Cl2. SO3: reacts with H2O. SO3/pyridine: sol DMSO; reacts with H2O. Form Supplied in: DMSO is a colorless liquid; SO3 is a low-boiling liquid, and the SO3/pyridine complex is a crystalline solid; widely available, including SO3/pyridine complex and “anhydrous” grades of DMSO packed under N2. For the preparation of SO3/pyridine complex see Sulfur Trioxide–Pyridine. Preparative Method: the active oxidant, formulated as Me2S+OSO3−,2d is generated in situ by mixing DMSO and the SO3/pyridine complex. Purification: DMSO: distillation from CaH2 at 56–57 °C/5 mmHg2a or 83–85 °C/17 mmHg;2b storage over 3Å molecular sieves. Handling, Storage, and Precautions: Dimethyl Sulfoxide is readily absorbed through the skin and should always be handled with gloves in a fume hood; Sulfur Trioxide and SO3/pyridine are toxic and corrosive, and react strongly with H2O; reactions with DMSO form foul-smelling byproducts and should be carried out with good ventilation, and the waste byproducts and liquids used for washing should be treated with KMnO4 solution to oxidize volatile sulfur compounds; DMSO undergoes appreciable disproportionation to dimethyl sulfide and dimethyl sulfone above 90 °C.2c

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.002
metaresearch head score (Gemma)0.002
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Not applicable · Consensus signal: none
GenreCandidate signal: Other · Consensus signal: none
Teacher disagreement score0.092
Threshold uncertainty score0.309

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0020.002
Meta-epidemiology (narrow)0.0060.002
Meta-epidemiology (broad)0.0040.001
Bibliometrics0.0030.003
Science and technology studies0.0020.001
Scholarly communication0.0010.001
Open science0.0060.002
Research integrity0.0010.005
Insufficient payload (model declined to judge)0.0920.113

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.012
GPT teacher head0.247
Teacher spread0.235 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designNot applicable
Domainnot available
GenreOther

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations1
Published2001
Admission routes1
Has abstractyes

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