Green‐Engineered All‐Substrate Mesoporous TiO<sub>2</sub> Photoanodes with Superior Light‐Harvesting Structure and Performance
Why this work is in the frame
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Bibliographic record
Abstract
Electrophoretic deposition (EPD) is employed successfully in a suspension of multicomponent TiO2 nanoparticulates of different sizes and morphologies to engineer a very robust bifunctional electrode structure for dye-sensitized solar cell (DSSC) applications that shows excellent light-harvesting and photoelectrochemical performance. Aqueous-synthesized anatase nanocrystallites and sub-micrometer-sized "sea urchin"-like rutile aggregates are formulated in a stable isopropanol suspension without resorting to binders or charging agents. Interestingly, extremely robust films are obtained because of the high surface reactivity, electrophoretic mobility, and unique morphology of the rutile aggregates. DSSCs built with the newly configured bifunctional electrode yielded a record efficiency (8.59 %) for EPD-fabricated devices without resorting to mechanical compression. Such green-engineered mesoporous electrode structures can be built on both metallic and plastic substrates and can find applications in various energy and environmental fields.
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Full frame distilled prediction
Teacher imitationNot calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.
Codex and Gemma teacher scores by category
| Category | Codex | Gemma |
|---|---|---|
| Metaresearch | 0.000 | 0.000 |
| Meta-epidemiology (narrow) | 0.000 | 0.000 |
| Meta-epidemiology (broad) | 0.000 | 0.000 |
| Bibliometrics | 0.000 | 0.000 |
| Science and technology studies | 0.000 | 0.000 |
| Scholarly communication | 0.000 | 0.000 |
| Open science | 0.000 | 0.000 |
| Research integrity | 0.000 | 0.000 |
| Insufficient payload (model declined to judge) | 0.000 | 0.000 |
Machine scores (provisional)
The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.
Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.
score_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it