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Record W2115160671 · doi:10.1139/v01-168

2000 Maxxam Award Lecture Unified theory of extraction

2001· article· en· W2115160671 on OpenAlexfundvenueno aff
Janusz Pawliszyn

Bibliographic record

VenueCanadian Journal of Chemistry · 2001
Typearticle
Languageen
FieldChemistry
TopicAnalytical chemistry methods development
Canadian institutionsnot available
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsExtraction (chemistry)Process (computing)Process engineeringMass transferChemistryAutomationMatrix (chemical analysis)Computer scienceBiological systemChromatographyMechanical engineering

Abstract

fetched live from OpenAlex

The sample preparation step in an analytical process typically consists of extraction of components of interest from a sample matrix. This procedure can vary in degree of selectivity, speed, and convenience depending on the approach and conditions used as well as on geometric configurations of the extraction phase and conditions. Optimization of this process aids enhancement in performance of the overall analysis. Proper design of the extraction devices and procedures facilitates rapid and convenient on-site implementation, coupling to separation–quantification, and (or) automation. The key to rational choice, optimization, and design is an understanding of fundamental principles governing mass transfer of analytes in multiphase systems. There is a tendency to divide extraction techniques according to random criteria. In this article, common principles among different extraction techniques are emphasized and a unified approach based on convolution of mathematical functions describing individual steps is presented. This approach considers gas, solvent, liquid polymer, and solid surfaces as extraction phases and air, water, and solids as sample matrices. The parameters that affect the kinetics of extraction techniques are emphasized resulting in new calibration strategies and novel geometric designs.Key words: separations, extractions, microextractions, mass transfer, multiphase equilibria.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.001
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.188
Threshold uncertainty score0.988

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0130.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.020
GPT teacher head0.260
Teacher spread0.240 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations8
Published2001
Admission routes2
Has abstractyes

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