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Record W2123328146 · doi:10.1002/qua.21120

Nonequilibrium dynamics of single polymer molecules: Relaxation close to and far from equilibrium

2006· article· en· W2123328146 on OpenAlexafffund
Felix Hanke, H. J. Kreuzer

Bibliographic record

VenueInternational Journal of Quantum Chemistry · 2006
Typearticle
Languageen
FieldPhysics and Astronomy
TopicForce Microscopy Techniques and Applications
Canadian institutionsDalhousie University
FundersKillam Trusts
KeywordsNon-equilibrium thermodynamicsRelaxation (psychology)Master equationExponential functionMoleculeStatistical physicsExponential decayQuantumPolymerChemistryFokker–Planck equationAutocatalytic reactionPhysicsThermodynamicsQuantum mechanicsNuclear magnetic resonanceMathematicsDifferential equation

Abstract

fetched live from OpenAlex

Abstract A master equation approach is used to study the relaxation of single polymer molecules. For relaxation close to equilibrium, a Fokker–Planck equation is derived via a Kramers–Moyal expansion. Far from equilibrium, two scenarios are studied: (i) an initial force that stretched the molecule to a certain length is suddenly released and the time evolution to the final force‐free equilibrium is followed; and (ii) a force of a certain magnitude is suddenly applied to a molecule and the time evolution to the final equilibrium stretching at that force is followed. Initial transients, dominated by many time scales, are followed by a roughly exponential decay. Final approach to equilibrium is again exponential, but on a time scale many orders of magnitude slower. © 2006 Wiley Periodicals, Inc. Int J Quantum Chem, 2006

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.046
Threshold uncertainty score0.408

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.006
GPT teacher head0.252
Teacher spread0.247 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations5
Published2006
Admission routes2
Has abstractyes

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