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Rotational and Translational Dynamics in Solids

2009· reference-entry· en· W2125160199 on OpenAlexaff
Christopher I. Ratcliffe

Bibliographic record

VenueEncyclopedia of Magnetic Resonance · 2009
Typereference-entry
Languageen
FieldChemistry
TopicAdvanced NMR Techniques and Applications
Canadian institutionsNational Research Council Canada
Fundersnot available
KeywordsRotational dynamicsDynamics (music)PhysicsStatistical physicsChemistryQuantum mechanics

Abstract

fetched live from OpenAlex

The interactions between atoms, molecules, and ions ultimately determine the structural forms of solid materials, and in turn the crystal structure itself imposes potential fields around these components, which strongly influence their dynamic behavior in the solid. This article discusses the many ways in which solid-state NMR has been used to explore this intimate connection between crystal structure and dynamics, emphasizing how the interplay between crystal and molecular symmetry affects translational and rotational motions. Brief descriptions of theory are given and different aspects are highlighted with examples. NMR studies of dynamics can yield structural information which is complementary to diffraction data, such as internuclear distances, angles between rotational and crystal axes, and symmetry information. In a number of instances, such information has been used to improve or direct structural refinements, especially where there are problems of disorder. NMR gives aspects of local structure and is sensitive to dynamics on various timescales, in contrast with diffraction, which gives a long-range spatial average of electron density with little or no temporal information. NMR also provides a wealth of other information, including activation energies required to cross barriers, rotational rates or correlation times, and dynamic behavior around phase transitions.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Other design · Consensus signal: none
GenreCandidate signal: Other · Consensus signal: none
Teacher disagreement score0.980
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.009
GPT teacher head0.261
Teacher spread0.252 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designOther design
Domainnot available
GenreOther

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations1
Published2009
Admission routes1
Has abstractyes

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