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Record W2133132574 · doi:10.1002/apj.5500100108

Optimisation of Methyl Tert‐Butyl‐Ether (MTBE) Synthesis Processes using Aspen‐Plus

2002· article· en· W2133132574 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueDevelopments in Chemical Engineering and Mineral Processing · 2002
Typearticle
Languageen
FieldEngineering
TopicProcess Optimization and Integration
Canadian institutionsUniversity of Waterloo
Fundersnot available
KeywordsReactive distillationDistillationExtractive distillationProcess engineeringEffluentIsothermal processFractionating columnChemistryEnvironmental scienceThermodynamicsChromatographyEngineeringEnvironmental engineeringPhysics

Abstract

fetched live from OpenAlex

Abstract Four different configurations for the production of MTBE were simulated and optimised using AspenPlus All process configurations were simulated and costed using AspenPlus The total annual cost (TAC), i e the sum of the individual annualised capital and operating costs, was calculated using models consistent with the conceptual design level Optimisation of each process configuration using AspenPlus simulation models was performed to determine the optimal design and operating variables The optimised configurations were compared on an economic basis It was possible to achieve iso‐butylene conversions in the range of 90 to 97% with a single conventional reactor followed by a distillation tower However, by using a reactive distillation column it was possible to achieve iso‐butylene conversions > 99% The optimal configuration was found to be a combination of an isothermal reactor followed by a catalytic distillation column The optimal TAC of this configuration was 22% lower than its nearest competitor, the catalytic distillation column It was found that the net MTBE reaction rate remains high until a substantial amount of iso‐butylene is converted, and then decreases quickly as the reacting liquid composition approaches the reaction equilibrium Therefore, it is not surprising that the best means of synthesis is to carry out the bulk of the initial conversion using a conventional reactor and to apply reactive distillation to the reactor effluent that is close to equilibrium at the exit temperature

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Simulation or modeling · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.271
Threshold uncertainty score0.853

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.021
GPT teacher head0.219
Teacher spread0.198 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it