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Nickel Isotope Variations in Terrestrial Silicate Rocks and Geological Reference Materials Measured by <scp>MC</scp>‐<scp>ICP</scp>‐<scp>MS</scp>

2013· article· en· W2133650956 on OpenAlexafffund
Bleuenn Guéguen, Olivier Rouxel, Emmanuel Ponzevera, Andrey Bekker, Yves Fouquet

Bibliographic record

VenueGeostandards and Geoanalytical Research · 2013
Typearticle
Languageen
FieldEarth and Planetary Sciences
TopicPaleontology and Stratigraphy of Fossils
Canadian institutionsUniversity of Manitoba
FundersNatural Sciences and Engineering Research Council of CanadaInstitut Français de Recherche pour l'Exploitation de la Mer
KeywordsIsotopeSilicateGeologyIgneous rockMineralogyGeochemistryAnalytical Chemistry (journal)ChemistryMass spectrometryEnvironmental chemistryChromatography

Abstract

fetched live from OpenAlex

Although initial studies have demonstrated the applicability of N i isotopes for cosmochemistry and as a potential biosignature, the N i isotope composition of terrestrial igneous and sedimentary rocks, and ore deposits remains poorly known. Our contribution is fourfold: (a) to detail an analytical procedure for N i isotope determination, (b) to determine the N i isotope composition of various geological reference materials, (c) to assess the isotope composition of the B ulk S ilicate E arth relative to the N i isotope reference material NIST SRM 986 and (d) to report the range of mass‐dependent N i isotope fractionations in magmatic rocks and ore deposits. After purification through a two‐stage chromatography procedure, N i isotope ratios were measured by MC ‐ ICP ‐ MS and were corrected for instrumental mass bias using a double‐spike correction method. Measurement precision (two standard error of the mean) was between 0.02 and 0.04‰, and intermediate measurement precision for NIST SRM 986 was 0.05‰ (2 s ). Igneous‐ and mantle‐derived rocks displayed a restricted range of δ 60/58 N i values between −0.13 and +0.16‰, suggesting an average BSE composition of +0.05‰. Manganese nodules (Nod A1; P1), shale ( SDO ‐1), coal ( CLB ‐1) and a metal‐contaminated soil ( NIST SRM 2711) showed positive values ranging between +0.14 and +1.06‰, whereas komatiite‐hosted N i‐rich sulfides varied from −0.10 to −1.03‰.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.005
metaresearch head score (Gemma)0.011
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMetaresearch, Meta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Observational · Consensus signal: Observational
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.117
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0050.011
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.001
Science and technology studies0.0010.001
Scholarly communication0.0010.001
Open science0.0010.000
Research integrity0.0010.001
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.052
GPT teacher head0.306
Teacher spread0.255 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designObservational
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations127
Published2013
Admission routes2
Has abstractyes

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