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Record W2136906725 · doi:10.1039/c3tb20391c

A nanocomposite contact lens for the delivery of hydrophilic protein drugs

2013· article· en· W2136906725 on OpenAlexaff
Jin Zhang, Robert Bi, William Hodge, Pei Yin, Wai Hei Tse

Bibliographic record

VenueJournal of Materials Chemistry B · 2013
Typearticle
Languageen
FieldMedicine
TopicOcular Surface and Contact Lens
Canadian institutionsWestern University
Fundersnot available
KeywordsGelatinMethacrylateContact lensNanocompositeSwellingMaterials scienceBovine serum albuminSelf-healing hydrogelsControlled releaseDrug delivery(Hydroxyethyl)methacrylateCopolymerContact anglePolymer chemistryChemical engineeringChemistryChromatographyNanotechnologyComposite materialOrganic chemistryPolymerOphthalmologyMedicine

Abstract

fetched live from OpenAlex

To improve the efficiency of topical ocular drug administration, we developed a nanocomposite contact lens to deliver hydrophilic protein drugs over a prolonged period of time. Here, an in situ route was used to encapsulate the hydrophilic protein drug bovine serum albumin (BSA) within gelatin nanoparticles (NPs), 180 ± 20 nm in diameter, which were then grafted onto the lens material, a copolymer of 2-hydroxyethyl methacrylate and 2-aminoethyl methacrylate p(HEMA-co-AEMA), through photopolymerization. The thickness of the nanocomposite lens was controlled at 150 μm. The release kinetics of BSA from plain p(HEMA-co-AEMA), gelatin NPs, and gelatin NP-grafted p(HEMA-co-AEMA) in phosphate buffer saline (PBS) at pH = 7.4 were studied. The release profile of BSA encapsulated within gelatin NPs could be monitored for 7 days, three times longer than that of BSA soaked in p(HEMA-co-AEMA). Our findings indicate that use of the nanocomposite contact lens, i.e. BSA-loaded gelatin NPs incorporated into p(HEMA-co-AMEA), can prolong the release profile of BSA to 12 days. The swelling behavior and interior strain of p(HEMA-co-AEMA) with and without grafted NPs (1000 : 1 w/w) were further investigated. The nanocomposite lens shows higher swelling behavior than the plain p(HEMA-co-AEMA) lens does. The addition of gelatin NPs to hydrogels leads to a relatively uniform interior strain with lower stiffness. Thus, the prolonged release might be due to a combination of effects. Internal diffusion of the nanocomposite lens materials may significantly contribute to the prolonged release of protein drugs. Furthermore, the nanocomposite lens materials had no cytotoxicity. This new biocompatible nanocomposite might be further developed as an alternative tool for continuous topical ocular drug delivery over a prolonged period of time.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.005
Threshold uncertainty score0.518

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.009
GPT teacher head0.225
Teacher spread0.216 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations29
Published2013
Admission routes1
Has abstractyes

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