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Effects of supercritical CO2 on the viscosity and morphology of polymer blends

2000· article· en· W2140252179 on OpenAlexaff
Min‐Hee Lee, Costas Tzoganakis, Chul B. Park

Bibliographic record

VenueAdvances in Polymer Technology · 2000
Typearticle
Languageen
FieldMaterials Science
TopicPolymer Foaming and Composites
Canadian institutionsUniversity of TorontoUniversity of Waterloo
FundersLG Chem
KeywordsMaterials scienceSupercritical fluidPlastics extrusionExtrusionPolymerSupercritical carbon dioxidePolystyrenePolymer blendDissolutionViscosityComposite materialChemical engineeringMiscibilityPhase (matter)Polymer chemistryCopolymerOrganic chemistryChemistry

Abstract

fetched live from OpenAlex

Supercritical carbon dioxide (CO2) was used in extrusion for the improvement of polymer blend properties. Various extruder configurations using a twin-screw extruder and a single-screw extruder were designed for investigating the effects of dissolved supercritical CO2 on the viscosity and morphological properties of polyethylene, polystyrene, and their blends. The viscosities of the polymer/CO2 and the blend/CO2 solutions were measured at various concentrations of CO2 and PE/PS blending ratios using a wedge die mounted on the twin-screw extruder. The effect of CO2 on the morphology of PE/PS blends was also investigated using a twin/single-screw tandem system. This system allowed for preferential dissolution of the CO2 into the matrix and/or dispersed polymer phase. By introducing devolatilization to the tandem system, the morphological behaviors of PE/PS blends were investigated on unfoamed filaments. In general, the mixing between two polymers was improved by the dissolution of CO2. The size reduction of the dispersed phase was explained using the viscosity ratio of the two polymers. Finally, the interface between foamed and unfoamed polymers was studied in a bilayer structure produced by using a special configuration of the tandem system. © 2000 John Wiley & Sons, Inc. Adv Polym Techn 19: 300–311, 2000

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.003

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0010.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.003
GPT teacher head0.230
Teacher spread0.227 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations79
Published2000
Admission routes1
Has abstractyes

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