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Record W2140488032 · doi:10.5539/eer.v4n2p90

In-situ Decomposition of Trichloroethylene Using Electrochemical Treatment Method

2014· article· en· W2140488032 on OpenAlexvenueno aff
Takuya Ito, Kazuyuki Yamada, S. Kato, Hideki Suganuma, Akihiro Yamasaki, Seiichi Suzuki, Toshinori Kojima

Bibliographic record

VenueEnergy and Environment Research · 2014
Typearticle
Languageen
FieldEngineering
TopicElectrokinetic Soil Remediation Techniques
Canadian institutionsnot available
Fundersnot available
KeywordsTrichloroethyleneDecompositionEnvironmental remediationAqueous solutionContaminationElectrodeDegreasingSoil waterMaterials scienceElectrochemistryVolumetric flow rateChemical engineeringAqueous two-phase systemChemistryEnvironmental chemistryAnalytical Chemistry (journal)Environmental scienceComposite materialOrganic chemistrySoil scienceThermodynamics

Abstract

fetched live from OpenAlex

Trichloroethylene (TCE) has an excellent degreasing capacity, so it is often used as a solvent for dry cleaning, and is still used for removing grease from metallic parts and so on. However, its inappropriate handling caused contamination of soil. Recently, its toxicity and carcinogenicity to humans have been concerned. By these reasons, it is highly required to remediate the contaminated soils. In the present study, the possibility of application of electrochemical treatment method to the in-situ decomposition of TCE is examined because in-situ remediation is expected to be simple and inexpensive. The experiment in the aqueous systems was conducted as a basic examination. As a result of comparing experimental values under various stirring speeds with the theoretical value calculated from mass transfer coefficient, it turned out that TCE transferring from bulk to the electrode surface is accelerated by the radicals in the boundary film near the electrode surface. Hence the TCE decomposition rate is affected by the radical formation rate or radical concentration in the boundary film. In the experiment with the soils, the TCE decomposition rate was much smaller than that in the aqueous systems. Moreover, the influence of the voltage was not observed. Therefore, it turned out that the movement of TCE in the aqueous phase near the electrode surface was the rate-controlling step in the soils. Under the condition, the TCE decomposition rate was not affected by the particle size. Consequently, it turned out TCE is not transported by bulk flow but is mostly transfered by molecular diffusion in the soil.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.003

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.019
GPT teacher head0.317
Teacher spread0.298 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations2
Published2014
Admission routes1
Has abstractyes

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