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Lead Removal from Acidic Solutions by Sorption on Cocoa Shells: Effect of Some Parameters

2003· article· en· W2145681112 on OpenAlexaff
Nathalie Meunier, Jéro⁁me Laroulandie, Jean‐François Blais, R. D. Tyagi

Bibliographic record

VenueJournal of Environmental Engineering · 2003
Typearticle
Languageen
FieldEnvironmental Science
TopicAdsorption and biosorption for pollutant removal
Canadian institutionsInstitut National de la Recherche ScientifiqueInstitut National d'Optique
FundersU.S. Environmental Protection Agency
KeywordsSorptionChemistrySorbentNuclear chemistryIon exchangeLaboratory flaskAmine gas treatingIonAdsorptionOrganic chemistry

Abstract

fetched live from OpenAlex

The objectives of this work were to evaluate the effects of different parameters (Pb concentration, solution pH, Ca/Mg/Na/K salt concentrations) on Pb uptake by cocoa shells and to study the mechanisms of Pb removal in very acidic conditions. Sorption tests were conducted in shaken flasks with synthetic Pb solutions and 15 g/L cocoa shells. A lead uptake value of 161 mmol/kg was measured during the assay with [Pb]i=3.66 mmol/L in solution at pHi=2.0 and T=22°C. Results show that Pb uptake is very similar (14.5–16.0 mmol/kg) for an initial pH between 2.0 and 4.0, but a moderate decrease (10.8 mmol/kg) occurred when the initial pH=1.5 and the [Pb]i=0.25 mmol/L. High Ca and Mg concentrations (2.35 mol/L) in solution induced a significant decrease in Pb removal by cocoa shells, whereas high K and Na concentrations did not affect Pb uptake by this sorbent. This suggests that Pb uptake by cocoa shells is controlled by ion-exchange reactions with Ca/Mg ions and protons. Finally, chemical tests have shown that carboxyl and amine functional groups play a dominant role in Pb uptake by cocoa shells.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.005
Threshold uncertainty score0.010

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.007
GPT teacher head0.188
Teacher spread0.181 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations49
Published2003
Admission routes1
Has abstractyes

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