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Record W2236089490 · doi:10.1002/cjce.22369

Simultaneous CO<sub>2</sub>/SO<sub>2</sub> adsorption performance of carbide slag in adsorption/desorption cycles

2015· article· en· W2236089490 on OpenAlexvenueno aff
Shuimu Wu, Yingjie Li, Jianli Zhao, Chunmei Lu, Zeyan Wang

Bibliographic record

VenueThe Canadian Journal of Chemical Engineering · 2015
Typearticle
Languageen
FieldEngineering
TopicChemical Looping and Thermochemical Processes
Canadian institutionsnot available
FundersNational Natural Science Foundation of ChinaShandong University
KeywordsAdsorptionCarbonationDesorptionCarbideMaterials scienceSlag (welding)SorbentChemical engineeringMetallurgyParticle sizeChemistryComposite materialOrganic chemistry

Abstract

fetched live from OpenAlex

Abstract Simultaneous CO2/SO2 adsorption performance of CaO derived from carbide slag (an industrial waste product from a chlor‐alkali plant) in multiple adsorption/desorption cycles was investigated in a dual fixed‐bed reactor. The effects of adsorption duration, SO2 concentration, adsorption temperature, desorption conditions, and particle size on carbonation conversion, cumulative sulphation conversion, and total Ca utilization of the carbide slag over multiple cycles were discussed. SO2 presence appreciably impedes the cyclic CO2 adsorption capacity of the carbide slag. A longer adsorption duration causes a sharper drop in the carbonation conversion due to the adverse effect of SO2. The presence of SO2 intensifies the effect of adsorption temperature on the carbonation conversion of the carbide slag. The optimum adsorption temperature for cyclic simultaneous CO2/SO2 adsorption by the carbide slag is 700 °C. The high desorption temperature and CO2 concentration (950 °C, 0.9999 L/L CO2) are not beneficial to cyclic CO2/SO2 adsorption. Both the carbonation conversion and cumulative sulphation conversion of the carbide slag decrease with increasing sorbent particle size in the cycles. The compact CaSO4 product layer covers the surface of CaO derived from the carbide slag during the multiple cycles, which results in a sharp drop in the surface area and pore volume with the cycle number. Compared with limestone, the carbide slag exhibits higher SO2 adsorption capacity and similar CO2 adsorption capacity during the cyclic simultaneous CO2/SO2 adsorption.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.004
Threshold uncertainty score0.008

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.009
GPT teacher head0.191
Teacher spread0.182 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations33
Published2015
Admission routes1
Has abstractyes

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