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Record W2236864445

The Effects of Water Chemistry and Organism Source on Dysprosium Toxicity to Hyalella Azteca

2016· dissertation· en· W2236864445 on OpenAlexaboutno aff
Lu Che

Bibliographic record

VenueUWSpace (University of Waterloo) · 2016
Typedissertation
Languageen
FieldChemistry
TopicAnalytical chemistry methods development
Canadian institutionsnot available
Fundersnot available
KeywordsHyalella aztecaDysprosiumOrganismToxicityWater chemistryEnvironmental chemistryChemistryToxicologyEcologyBiologyInorganic chemistryAmphipodaCrustaceanOrganic chemistry
DOInot available

Abstract

fetched live from OpenAlex

Rare earth elements (REEs) are a series of seventeen chemical elements, containing mostly lanthanides. Due to their multiple applications in industry and consumer electronics, global demand and production of REE has been increasing. Canada has the potential to be one of the major REE producers, with reserves mainly located in northern regions, yet there is limited knowledge of the potential environmental impact of mining and refining of REEs. Dysprosium (Dy) is one of the most widely used heavy REEs due to its magnetic strength. In this study, acute 96 h toxicity tests were conducted to determine the sensitivity to Dy for four different sources (Fort Hope, Hannah Lake, Daisy Lake, Low Water Lake, ON) of Hyalella azteca as well as Daphnia pulex. LC50s and their confidence intervals derived from dissolved Dy concentrations indicated significant differences in Dy sensitivity as a function of the source of H. azteca. To determine the potential influence of toxicity modifying factors on Dy toxicity, acute (96 h) and chronic (28 d) toxicity tests using H. azteca were conducted with differing concentrations of Ca2+, Mg2+ and Na+ (acute test only), differing qualities and/or concentrations of dissolved organic carbon (DOC) as well as differing pH. Based on LC50 data for 96 h tests, Ca2+ (2 mM), Na+ (2 mM), low pH (6.7) and DOC (Suwannee River, USA; 9.6 mg/L), but not Mg2+ (up to 2 mM) demonstrated protective effects against Dy toxicity. In addition, pH played an important role in Dy solubility. For 28 d exposures, protective effects against Dy toxicity were demonstrated for Ca2+ (2 mM), Mg2+ (0.5 mM) and DOC (White River and Luther Marsh, ON; 6.4 and 7.8 mg/L respectively) based on dissolved Dy LC50s. Both types of DOC were found to partially ameliorate growth inhibition at low Dy concentrations. One of the sources of DOC (Luther Marsh) was very effective at reducing Dy bioaccumulation in H. azteca. The LC50 data for 96 h toxicity tests contributed to building a preliminary Dy biotic ligand model (BLM) of H. azteca, which will assist with estimations of Dy toxicity in aquatic systems that differ in water quality and provide knowledge to direct the establishment of water resource protection guidelines of REE in Canada.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.009
Threshold uncertainty score0.018

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0010.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.005
GPT teacher head0.196
Teacher spread0.191 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2016
Admission routes1
Has abstractyes

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