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Record W2259519747 · doi:10.1021/acs.jced.5b00710

Effect of the Presence of MEA on the CO<sub>2</sub> Capture Ability of Superbase Ionic Liquids

2016· article· en· W2259519747 on OpenAlex
Corina McCrellis, S. F. Rebecca Taylor, Johan Jacquemin, Christopher Hardacre

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

fundA Canadian funder is recorded on the work.
no affNo Canadian affiliation: this work is invisible to an affiliation-only frame.
No Canadian affiliation. An affiliation-only frame, the usual design, would never have seen this work. It is one of the works that make the case for inverting the frame.

Bibliographic record

VenueJournal of Chemical & Engineering Data · 2016
Typearticle
Languageen
FieldChemical Engineering
TopicIonic liquids properties and applications
Canadian institutionsnot available
FundersEngineering and Physical Sciences Research CouncilQueen's UniversityUniversity College LondonQueen's University BelfastDepartment for Employment and Learning, Northern Ireland
KeywordsChemistryIonic liquidSuperbaseGravimetric analysisMiscibilitySolubilityThermodynamicsPhysical chemistryOrganic chemistry

Abstract

fetched live from OpenAlex

High Resolution Image Download MS PowerPoint Slide The miscibility of monoethanolamine (MEA) in five superbase ionic liquids (ILs), namely the trihexyl-tetradecylphosphonium benzotriazolide ([P 66614 ][Bentriz]), trihexyl-tetradecylphosphonium benzimidazolide ([P 66614 ][Benzim]), trihexyl-tetradecylphosphonium 1,2,3-triazolide ([P 66614 ][123Triz]), trihexyl-tetradecylphosphonium 1,2,4-triazolide ([P 66614 ][124Triz]), and trihexyl-tetradecylphosphonium imidazolide ([P66614][Im]) was determined at 295.15 K using 1 H NMR spectroscopy. The solubility of carbon dioxide (CO 2 ) in equimolar (IL + MEA) mixtures was then studied experimentally using a gravimetric technique at 295.15 K and 0.1 MPa. The effect of MEA on the CO 2 capture ability of these ILs was investigated together with the viscosity of these systems in the presence or absence of CO 2 to evaluate their practical application in CO 2 capture processes. The effect of the presence of MEA on the rate of CO 2 uptake was also studied. The study showed that the MEA can enhance CO 2 absorption over the ideal values in the case of [P 66614 ][123Triz] and [P 66614 ][Bentriz] while in the other systems the mixtures behave ideally. A comparison of the effect of MEA addition with the addition of water to these superbase ILs showed that similar trends were observed in each case for the individual ILs studied.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.002
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.004
Threshold uncertainty score0.289

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.002
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.013
GPT teacher head0.234
Teacher spread0.222 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it