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Stabilization of Polypropylene for Rotational Molding Applications

2016· article· en· W2271385461 on OpenAlex
Iñaki Emaldi, Christopher M. Liauw, J.H. Potgieter

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

venuePublished in a venue whose home country is Canada.
no affNo Canadian affiliation: this work is invisible to an affiliation-only frame.
No Canadian affiliation. An affiliation-only frame, the usual design, would never have seen this work. It is one of the works that make the case for inverting the frame.

Bibliographic record

VenueJournal of Research Updates in Polymer Science · 2016
Typearticle
Languageen
FieldMaterials Science
TopicPolymer crystallization and properties
Canadian institutionsnot available
FundersManchester Metropolitan University
KeywordsPolypropyleneMaterials scienceMolding (decorative)AntioxidantComposite materialToughnessPolyethyleneCopolymerCompression moldingAmine gas treatingPrimary (astronomy)Melt flow indexYield (engineering)Stabilizer (aeronautics)PolymerChemical engineeringPolymer chemistryOrganic chemistryChemistryMechanical engineering

Abstract

fetched live from OpenAlex

Rotational molding (RM) is a useful process for making large hollow objects. Due to its relatively high toughness and forgiving thermal oxidative degradation behavior, polyethylene is a most widely used material. However, it has too low elastic modulus for some important applications which leads to adaptation of polypropylene (PP) as a RM material. PP requires specially tailored antioxidant (AO) packages if it is to have any chance of surviving the often long (up to ca. 30 minutes) cycle times associated with RM. During the study the addition of the following stabilizers and antioxidants (AO) to the PP copolymer were investigated: a hindered phenolic primary AO, a phosphite secondary AO, a thioester secondary AO and a hindered amine light stabilizer. Synergistic effects between the primary and secondary AOs, as well as optimum heating times, were investigated. During the investigation formulations were prepared by compression molding and bench-scale RM. The combination resulting in the most effective synergism is the hindered phenolic primary antioxidant combined with the phosphite secondary antioxidant. A gel silica controlled release agent for the stabilizers was also investigated but did not yield significant improvements in stabilization.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.005
metaresearch head score (Gemma)0.001
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.097
Threshold uncertainty score0.439

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0050.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0010.001
Science and technology studies0.0000.001
Scholarly communication0.0000.001
Open science0.0010.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.062
GPT teacher head0.394
Teacher spread0.332 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it