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Record W2314715478 · doi:10.1021/je200905z

High-Pressure Solubility of Methane (CH<sub>4</sub>) and Ethane (C<sub>2</sub>H<sub>6</sub>) in Mixed Polyethylene Glycol Dimethyl Ethers (Genosorb 1753) and Its Selectivity in Natural Gas Sweetening Operations

2012· article· en· W2314715478 on OpenAlex
Aravind V. Rayer, Amr Henni, Paitoon Tontiwachwuthikul

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueJournal of Chemical & Engineering Data · 2012
Typearticle
Languageen
FieldEngineering
TopicPhase Equilibria and Thermodynamics
Canadian institutionsUniversity of Regina
FundersClariant
KeywordsChemistryNon-random two-liquid modelSolubilityEnthalpyThermodynamicsGibbs free energyActivity coefficientHeat capacityMethaneOrganic chemistryAqueous solution

Abstract

fetched live from OpenAlex

The solubility of methane (CH 4 ) and ethane (C 2 H 6 ) in a mixture of polyethylene glycol dimethyl ethers (Genosorb 1753) was measured at (298.15, 313.15, and 333.15) K and at pressures up to 7700 kPa using a Jerguson equilibrium cell. The solubility data of CO 2 and light hydrocarbons (CH 4 and C 2 H 6 ) in Genosorb 1753 were compared with the solubility in other physical solvents. The results were correlated with the Peng–Robinson equation of state (PR-EOS), and the interaction parameters are reported. Among the activity coefficient models, the Non-Random Two Liquid Theory (NRTL) model fitted the data well with an absolute average deviation of 6 %. Henry’s Law constants ( H CH 4 and H C 2 H 6 ) and the excess properties (excess Gibbs free energy ( G E ), excess entropy ( S E ), and excess enthalpy ( H E )) of the liquid mixture were predicted at each temperature using the NRTL activity coefficient model over the full range of composition. The enthalpy of solution and the partial molar enthalpy of mixing for all gases were determined at infinite dilution. In addition, the enthalpies of solution for all the gases were calculated using the Clausius–Clapeyron equation. The coabsorption of hydrocarbons (CH 4 and C 2 H 6 ) with CO 2 (selectivity) was evaluated with the following function { H CO 2 /( H CH 4 · H C 2 H 6 )}. Compared to other solvents used in gas sweetening, Genosorb 1753 was found to have the highest absorption capacity for CO 2 and a low capacity for CH 4 but a higher capacity for C 2 H 6 .

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.001
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.153
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.001
Meta-epidemiology (narrow)0.0010.001
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.001
Open science0.0010.000
Research integrity0.0000.002
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.012
GPT teacher head0.228
Teacher spread0.216 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it