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Record W2314871231 · doi:10.1021/am404122v

Green-Sensitive Organic Photodetectors with High Sensitivity and Spectral Selectivity Using Subphthalocyanine Derivatives

2013· article· en· W2314871231 on OpenAlexaff
Kwanghee Lee, Dong‐Seok Leem, Jeffrey S. Castrucci, Kyung‐Bae Park, Xavier Bulliard, Kyu‐Sik Kim, Yong Jin, Sangyoon Lee, Timothy P. Bender, Soo Young Park

Bibliographic record

VenueACS Applied Materials & Interfaces · 2013
Typearticle
Languageen
FieldEngineering
TopicOrganic Electronics and Photovoltaics
Canadian institutionsUniversity of Toronto
Fundersnot available
KeywordsMaterials scienceFull width at half maximumQuantum efficiencySelectivityOptoelectronicsSpectral sensitivityPhotodetectorWavelengthAnalytical Chemistry (journal)OpticsChemistry

Abstract

fetched live from OpenAlex

Green-sensitive organic photodetectors (OPDs) with high sensitivity and spectral selectivity using boron subphthalocyanine chloride (SubPc) derivatives are reported. The OPDs composed of SubPc and dicyanovinyl terthiophene derivative (DCV3T) demonstrated the highest green-sensitivity with maximum external quantum efficiency (EQE) of 62.6 % at an applied voltage of -5 V, but wide full-width-at-half-maximum (FWHM) of 211 nm. The optimized performance considering spectral selectivity was achieved from the composition of N,N-dimethyl quinacridone (DMQA) and SubPc showing the high specific detectivity (D*) of 2.34 × 10(12) cm Hz(1/2)/W, the EQE value of 60.1% at -5 V, and narrow FWHM of 131 nm. In spite of the sharp absorption property of SubPc with the maximum wavelength (λmax) at 586 nm, the EQE spectrum showed favorable green-sensitivity characterized by smooth waveform with λmax at 560 nm, which is induced from the high reflectance of SubPc centered at 605 nm. The photoresponsivity of the OPD devices was found to be consistent with their absorptance. Optimized DMQA/SubPc device showed the lowest value of blue crosstalk (0.42) and moderate red crosstalk (0.37), suggesting its promising application as a green-sensitive OPD.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.003
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.006
GPT teacher head0.181
Teacher spread0.176 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations102
Published2013
Admission routes1
Has abstractyes

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