MétaCan
Menu
Back to cohort
Record W2319248628 · doi:10.1021/jp405754v

<i>In Situ</i> Fabrication of Nafion–Titanate Hybrid Electrolytes for High-Temperature Direct Ethanol Fuel Cell

2013· article· en· W2319248628 on OpenAlexaff
Bruno R. Matos, Roberta A. Isidoro, Elisabete I. Santiago, Marcelo Linardi, André S. Ferlauto, Ana C. Tavares, Fábio C. Fonseca

Bibliographic record

VenueThe Journal of Physical Chemistry C · 2013
Typearticle
Languageen
FieldEngineering
TopicFuel Cells and Related Materials
Canadian institutionsInstitut National de la Recherche Scientifique
Fundersnot available
KeywordsNafionMaterials scienceNanorodChemical engineeringProton exchange membrane fuel cellRaman spectroscopyNanocompositeTitanateElectrolyteTransmission electron microscopyNanotechnologyComposite materialElectrochemistryElectrodeCeramicChemistryFuel cellsPhysical chemistryOptics

Abstract

fetched live from OpenAlex

The synthesis and characterization of a novel Nafion-matrix nanocomposite by the in situ conversion of titania particles into titanate nanofilaments such as nanotubes and nanorods are reported. Titania nanoparticles grown inside Nafion hydrophilic domains were converted by a microwave-assisted hydrothermal reaction into the proton conducting titanate nanotubes and nanorods. Detailed characterization by Raman spectroscopy, X-ray diffraction, small-angle X-ray scattering, and transmission electron microscopy evidenced an intimate interaction between titanate nanostructures and the ionomer hydrophilic phase. The favored localization of such high aspect ratio nanofilaments in the ionic phase of Nafion has a marked impact on the properties of the composites. The experimental data showed enhanced mechanical stability at high temperature (∼130 °C) that was correlated to a strong temperature dependence of the proton conductivity in the same temperature range. Such properties contributed to a significant increase of the performance of direct ethanol fuel cells operating at high temperature (∼130 °C) using hybrid Nafion–titanate electrolytes compared to commercial Nafion.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.002

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.002
GPT teacher head0.178
Teacher spread0.176 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations23
Published2013
Admission routes1
Has abstractyes

Explore more

Same venueThe Journal of Physical Chemistry CSame topicFuel Cells and Related MaterialsFrench-language works237,207