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Record W2320678767 · doi:10.1021/ie402096h

Photocatalytic Performance of Titanium Dioxide Thin Films from Polymer-Encapsulated Titania

2013· article· en· W2320678767 on OpenAlexaff
Charles R. Gilmour, Ajay K. Ray, Jesse Zhu, Madhumita B. Ray

Bibliographic record

VenueIndustrial & Engineering Chemistry Research · 2013
Typearticle
Languageen
FieldEnergy
TopicTiO2 Photocatalysis and Solar Cells
Canadian institutionsWestern University
Fundersnot available
KeywordsPhotocatalysisTitanium dioxideCatalysisCalcinationMaterials scienceChemical engineeringAdsorptionPolymerMethylene blueTitaniumCoatingPorosityTitanium oxideComposite materialChemistryOrganic chemistryMetallurgy

Abstract

fetched live from OpenAlex

The performance of a proprietary catalyst (VN-TiO 2 ) was compared with standard P25 TiO 2 for removal of methylene blue in water using immobilized photocatalysis. Using a fiberglass disk as the support medium dip coated in the VN-TiO 2 solution and calcining, porous films with a high surface area (up to 109 m 2 /g) were produced without any modification. Although films formed with VN-TiO 2 on fiberglass disks had a reaction rate 50% lower than that of P25, the disks coated with VN-TiO 2 were mechanically robust in the reactor, compared to those coated with P25. The addition of only 15 wt % P25 in the VN-TiO 2 solution increased the reaction rate by 40%, while maintaining the mechanical stability. The reuse potential of both catalysts was tested, and the rates of deactivation were comparable for both catalysts. Deactivation occurred due to sustained adsorption of Methylene Blue intermediates, as well as a loss of active sites, because of heat treatment for reactivation. Low-priced fiberglass in combination with the easily impregnable polymer-encapsulated titania is a viable option for producing mechanically robust and uniform catalyst coating for immobilized photoreactors.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.002
Threshold uncertainty score0.005

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.041
GPT teacher head0.262
Teacher spread0.221 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations9
Published2013
Admission routes1
Has abstractyes

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