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Record W2323443752 · doi:10.1021/ef101435r

Forced and Diffusive Mass Transfer between Pentane and Athabasca Bitumen Fractions

2011· article· en· W2323443752 on OpenAlexafffund
Ardalan Sadighian, Mildred Becerra, Ala Bazyleva, John M. Shaw

Bibliographic record

VenueEnergy & Fuels · 2011
Typearticle
Languageen
FieldChemistry
TopicPetroleum Processing and Analysis
Canadian institutionsUniversity of Alberta
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsPentaneMass transferChemistryImpellerAsphaltDiffusionMass transfer coefficientThermodynamicsShear (geology)Analytical Chemistry (journal)Materials scienceChromatographyOrganic chemistryComposite material

Abstract

fetched live from OpenAlex

Forced and diffusive mass transfer between pentane and Athabasca bitumen fractions was investigated at 297 K. Mutual diffusion coefficients were obtained using a free diffusion technique, where time-dependent composition profiles were jointly fit to obtain composition-dependent values. Because the density difference between pentane and Athabasca bitumen is significant, the density gradient was accounted for explicitly in the data analysis. Forced mass-transfer measurements were made by placing a high shear impeller in the pentane-rich phase adjacent to the pentane−feedstock interface. Mass-transfer coefficients were evaluated independently on the basis of the movement of the interface with time and changes in the bulk composition of the well-mixed pentane-rich phase above the interface. Because bitumen fractions are only partially soluble in pentane, the impact of the asymptotic assumptions, complete miscibility and complete immiscibility, on mass-transfer coefficient values obtained was assessed and found to fall within experimental error. The dependence of mass-transfer coefficients upon the shear rate and impeller-interface distance was also evaluated. Mass-transfer rates are shown to range from the diffusion limit at low shear rates and large impeller-interface distances to values consistent with those obtained from pertinent correlations for forced mass transfer under turbulent conditions at higher shear rates. The results suggest that bitumen−pentane mass transfer in reservoirs and surface facilities is likely to be diffusion-limited.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.003
Threshold uncertainty score0.007

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.001
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0020.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.016
GPT teacher head0.220
Teacher spread0.204 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations14
Published2011
Admission routes2
Has abstractyes

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