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Record W2323444365 · doi:10.1021/ef301866e

Determination of Multiphase Boundaries and Swelling Factors of Solvent(s)–CO<sub>2</sub>–Heavy Oil Systems at High Pressures and Elevated Temperatures

2013· article· en· W2323444365 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueEnergy & Fuels · 2013
Typearticle
Languageen
FieldEngineering
TopicPhase Equilibria and Thermodynamics
Canadian institutionsUniversity of Regina
Fundersnot available
KeywordsSolventThermodynamicsSwellingChemistrySaturation (graph theory)LogarithmPhase (matter)Equation of stateExponential functionFlory–Huggins solution theoryAnalytical Chemistry (journal)Materials scienceChromatographyMathematicsOrganic chemistryPhysics

Abstract

fetched live from OpenAlex

A generalized methodology has been proposed and successfully applied to determine multiphase boundaries as well as swelling factors of solvent(s)–CO 2 –heavy oil systems at high pressures and elevated temperatures. Experimentally, two- and three-phase boundaries and swelling factors have been respectively measured by conducting PVT tests in the temperature range of 280.45 to 396.15 K. Theoretically, the Peng–Robinson equation of state (PR EOS) combined with the modified alpha function has been applied to describe phase behavior of the solvent(s)–CO 2 –heavy oil systems. More specifically, an exponential distribution function is used to split a heavy oil sample, whereas the logarithm-type lumping method is employed to group single carbon numbers (SCNs) into multiple carbon numbers (MCNs). The exponents associated with two binary interaction parameter (BIP) correlations are respectively tuned for the alkane solvent-pseudocomponent pair and CO 2 -pseudocomponent pair to match the measured saturation pressures. It is found that six pseudocomponents combined with the BIP correlation as a function of critical volume is sufficient to predict saturation pressure with an absolute average relative deviation (AARD) of 5.07%. In addition, the PR EOS model associated with the selected parameters is applied to predict three-phase boundaries for a C 3 H 8 –CO 2 –heavy oil mixture and a n -C 4 H 10 –CO 2 –heavy oil mixture yielding an overall AARD of 4.58%. As for swelling factors, the Peneloux et al. method provides the minimum AARD of 2.09% in comparison with 4.00% from the Jhaveri et al. method and 2.41% from the Twu et al. method, respectively.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.040
Threshold uncertainty score0.723

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.006
GPT teacher head0.195
Teacher spread0.189 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it