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Record W2323444365 · doi:10.1021/ef301866e

Determination of Multiphase Boundaries and Swelling Factors of Solvent(s)–CO<sub>2</sub>–Heavy Oil Systems at High Pressures and Elevated Temperatures

2013· article· en· W2323444365 on OpenAlexaff
Xiaoli Li, Huazhou Li, Daoyong Yang

Bibliographic record

VenueEnergy & Fuels · 2013
Typearticle
Languageen
FieldEngineering
TopicPhase Equilibria and Thermodynamics
Canadian institutionsUniversity of Regina
Fundersnot available
KeywordsSolventThermodynamicsSwellingChemistrySaturation (graph theory)LogarithmPhase (matter)Equation of stateExponential functionFlory–Huggins solution theoryAnalytical Chemistry (journal)Materials scienceChromatographyMathematicsOrganic chemistryPhysics

Abstract

fetched live from OpenAlex

A generalized methodology has been proposed and successfully applied to determine multiphase boundaries as well as swelling factors of solvent(s)–CO 2 –heavy oil systems at high pressures and elevated temperatures. Experimentally, two- and three-phase boundaries and swelling factors have been respectively measured by conducting PVT tests in the temperature range of 280.45 to 396.15 K. Theoretically, the Peng–Robinson equation of state (PR EOS) combined with the modified alpha function has been applied to describe phase behavior of the solvent(s)–CO 2 –heavy oil systems. More specifically, an exponential distribution function is used to split a heavy oil sample, whereas the logarithm-type lumping method is employed to group single carbon numbers (SCNs) into multiple carbon numbers (MCNs). The exponents associated with two binary interaction parameter (BIP) correlations are respectively tuned for the alkane solvent-pseudocomponent pair and CO 2 -pseudocomponent pair to match the measured saturation pressures. It is found that six pseudocomponents combined with the BIP correlation as a function of critical volume is sufficient to predict saturation pressure with an absolute average relative deviation (AARD) of 5.07%. In addition, the PR EOS model associated with the selected parameters is applied to predict three-phase boundaries for a C 3 H 8 –CO 2 –heavy oil mixture and a n -C 4 H 10 –CO 2 –heavy oil mixture yielding an overall AARD of 4.58%. As for swelling factors, the Peneloux et al. method provides the minimum AARD of 2.09% in comparison with 4.00% from the Jhaveri et al. method and 2.41% from the Twu et al. method, respectively.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.002

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0010.000
Science and technology studies0.0000.001
Scholarly communication0.0000.001
Open science0.0000.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.006
GPT teacher head0.195
Teacher spread0.189 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations87
Published2013
Admission routes1
Has abstractyes

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