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Record W2325222522 · doi:10.1021/ie000215h

High-Temperature Conductivity Measurements for Industrial Applications. 2. H<sub>2</sub>SO<sub>4</sub>−Al<sub>2</sub>(SO<sub>4</sub>)<sub>3</sub> Solutions

2000· article· en· W2325222522 on OpenAlexaff
Morteza Baghalha, Vladimiros G. Papangelakis

Bibliographic record

VenueIndustrial & Engineering Chemistry Research · 2000
Typearticle
Languageen
FieldChemical Engineering
TopicChemical and Physical Properties in Aqueous Solutions
Canadian institutionsUniversity of Toronto
Fundersnot available
KeywordsMolalityConductivityChemistryIonic conductivityDrop (telecommunication)Analytical Chemistry (journal)Ionic bondingThermodynamicsElectrolyteInorganic chemistryIonAqueous solutionPhysical chemistryChromatography

Abstract

fetched live from OpenAlex

A new conductivity cell, developed previously, was employed from 15 to 250 °C, in an effort to investigate the inter-relation between the measured conductivities and the solution chemistry of high-temperature H 2 SO 4 −Al 2 (SO 4 ) 3 solutions. These electrolytes exist in the laterite leach slurry of the pressure acid leaching process. It was found that, at 250 °C, the effect of Al 2 (SO 4 ) 3 on conductivity decreases with increasing Al 2 (SO 4 ) 3 . This is in agreement with our previous findings that aluminum mostly forms Al(SO 4 ) + at low molalities, whereas 85% of aluminum is associated as Al 2 (SO 4 ) 3 0 at near-saturation molalities. At 250 °C and constant H 2 SO 4 molality, the solution conductivity drops with increasing Al 2 (SO 4 ) 3 molality. It is suggested that this drop is caused by a sharp decrease in ionic equivalent conductivities of H +, HSO 4 -, and Al(SO 4 ) + . This drop was found to be similar in nature to the drop when H 2 SO 4 is added at very low concentrations. A new unified correlation for ionic equivalent conductivity in terms of one-third power of individual ionic strength was found. Finally, a simple mixing rule was developed to calculate the ionic equivalent conductivities in H 2 SO 4 −Al 2 (SO 4 ) 3 solutions.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.002
metaresearch head score (Gemma)0.004
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Science and technology studies, Research integrity
Consensus categoriesMeta-epidemiology (narrow), Research integrity
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.034
Threshold uncertainty score0.999

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0020.004
Meta-epidemiology (narrow)0.0020.002
Meta-epidemiology (broad)0.0020.001
Bibliometrics0.0000.004
Science and technology studies0.0020.001
Scholarly communication0.0010.001
Open science0.0020.001
Research integrity0.0040.010
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.091
GPT teacher head0.289
Teacher spread0.199 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; both teacher heads agree on what is shown here.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations7
Published2000
Admission routes1
Has abstractyes

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