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Record W2325413701 · doi:10.1021/jp308418x

Insights into the Mechanism Related to the Phase Transition from γ-Fe<sub>2</sub>O<sub>3</sub> to α-Fe<sub>2</sub>O<sub>3</sub> Nanoparticles Induced by Thermal Treatment and Laser Irradiation

2012· article· en· W2325413701 on OpenAlexfundno aff
Yassine El Mendili, Jean‐François Bardeau, N. Randrianantoandro, Fabien Grasset, Jean−Marc Grenèche

Bibliographic record

VenueThe Journal of Physical Chemistry C · 2012
Typearticle
Languageen
FieldEnergy
TopicIron oxide chemistry and applications
Canadian institutionsnot available
FundersInstitute of Circulatory and Respiratory Health
KeywordsRaman spectroscopyMaterials scienceCrystalliteNanoparticleHematitePhase transitionAnnealing (glass)Powder diffractionIrradiationAnalytical Chemistry (journal)Thermal treatmentChemical engineeringCrystallographyNanotechnologyChemistryThermodynamicsOpticsMetallurgyComposite materialOrganic chemistry

Abstract

fetched live from OpenAlex

The nature of the physical mechanisms related to the γ-Fe 2 O 3 to α-Fe 2 O 3 phase transition under laser irradiation and heat treatment has been investigated using in situ micro-Raman spectroscopy and X-ray powder diffraction (XRPD) analysis. Measurements were carried out on as-prepared γ-Fe 2 O 3 nanoparticles of about 4 nm in size as a function of laser power and on annealed γ-Fe 2 O 3 particles. Annealing temperature affects the relative fractions of the γ-Fe 2 O 3 and α-Fe 2 O 3 phases, and at 450 °C, the phase transition into α-Fe 2 O 3 becomes complete with apparent crystallite size ⟨ D ⟩ of about 30 nm. The hematite nanoparticles increase then up to more than 180 nm at 1400 °C. The excellent agreement between evolution of the wavenumbers and bandwidths confirms that the heat treatment and laser irradiation produces the same effects on nanoparticles. Correlations between structure modifications occurring at the nanometric scale during grain coalescence and the evolution of Raman vibrational spectra were quantitatively examined, and a physical mechanism for the γ → α-Fe 2 O 3 phase transition was proposed.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.019
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.001
Science and technology studies0.0010.000
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.009
GPT teacher head0.231
Teacher spread0.221 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations120
Published2012
Admission routes1
Has abstractyes

Explore more

Same venueThe Journal of Physical Chemistry CSame topicIron oxide chemistry and applicationsFrench-language works237,207