A New Approach Towards Controlled Synthesis of Multifunctional Core–Shell Nano-Architectures: Luminescent and Superparamagnetic
Bibliographic record
Abstract
We have developed a two-step method for synthesis of multifunctional core-shell nanoparticles with an improved structure as compared with those prepared by traditional methods used independently. The nanoparticles comprise a superparamagnetic core, an inner insulating dye-free silica shell, an outer luminescent silica shell encapsulating thousands of dye molecules and a functionalizeable surface. The innovative insertion of the isolating silica shell benefits the nanoparticles' architecture in two ways. Firstly, by keeping the dye molecules away from the magnetic core, the silica shell prevents dye luminescence quenching. Secondly, the non-magnetic shell decreases magnetic interparticle coupling, which, by reducing aggregation and preventing agglomeration, facilitates the formation of the high-quality luminescent shell in the second step of the process. The final nanoparticles being both superparamagnetic and luminescent have a great potential for theranostic applications such as ultra-sensitive detection, and in-vitro and in-vivo imaging.
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How this classification was reachedexpand
Full frame distilled prediction
Teacher imitationNot calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.
Codex and Gemma teacher scores by category
| Category | Codex | Gemma |
|---|---|---|
| Metaresearch | 0.001 | 0.000 |
| Meta-epidemiology (narrow) | 0.000 | 0.000 |
| Meta-epidemiology (broad) | 0.001 | 0.000 |
| Bibliometrics | 0.000 | 0.000 |
| Science and technology studies | 0.000 | 0.001 |
| Scholarly communication | 0.000 | 0.000 |
| Open science | 0.000 | 0.000 |
| Research integrity | 0.000 | 0.000 |
| Insufficient payload (model declined to judge) | 0.000 | 0.000 |
Machine scores (provisional)
The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.
Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.
score_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from itClassification
machine, unvalidatedMachine predicted; a candidate call from one teacher head, not a consensus.
How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".