MétaCan
Menu
Back to cohort
Record W2330731088 · doi:10.1021/ef200681f

Asphaltene-Rich Phase Compositions and Sediment Volumes from Drying Experiments

2011· article· en· W2330731088 on OpenAlexafffund
Harvey W. Yarranton, F. S. Schoeggl, Simon C. George, Shawn D. Taylor

Bibliographic record

VenueEnergy & Fuels · 2011
Typearticle
Languageen
FieldChemistry
TopicPetroleum Processing and Analysis
Canadian institutionsSchlumberger (Canada)University of Calgary
FundersNatural Sciences and Engineering Research Council of CanadaPetrobrasUniversity of AlbertaSyncrude
KeywordsAsphalteneTolueneHeptaneSolventPentaneChemistryHildebrand solubility parameterSolubilityPhase (matter)EvaporationChemical engineeringChromatographyOrganic chemistryThermodynamics

Abstract

fetched live from OpenAlex

Drying experiments were performed on asphaltene sediments obtained from n-alkane diluted bitumen and asphaltenes precipitated from solutions of toluene and an n-alkane. The diffusive evaporation from within the asphaltene particles (asphaltene-rich phase) is much slower than free solvent evaporation, and in theory, the amount of solvent in the asphaltene-rich phase can be determined from a change in the evaporation rate. In practice, the evaporation of solvent within the asphaltene-rich phase could not be distinguished from the evaporation of a discontinuous film around the particles. Therefore, the measured solvent contents represent an upper limit to the solvent in the asphaltene-rich phase. The solvent contents of the asphaltene-rich phases from n-heptane diluted bitumen and solutions of toluene and n-heptane ranged from 6.5 to 8 wt %. The solvent contents of different asphaltene solubility cuts were within the ±1 wt % repeatability of the experiments. The extent of washing of the sediment also had no significant effect on the solvent content. The n-pentane content of the asphaltene-rich phase from n-pentane diluted bitumen was approximately 4 wt %, consistent with the lower solubility of asphaltenes in pentane relative to heptane. The drying experiments also demonstrated that the sediment became rigid at solvent contents of approximately 85 wt % equivalent to a porosity of approximately 90%. In other words, an asphaltene deposit may have a volume 10 times larger than the volume of the asphaltenes themselves.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.002
Threshold uncertainty score0.008

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0010.001
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0010.001
Science and technology studies0.0010.000
Scholarly communication0.0000.001
Open science0.0000.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0020.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.025
GPT teacher head0.265
Teacher spread0.240 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations7
Published2011
Admission routes2
Has abstractyes

Explore more

Same venueEnergy & FuelsSame topicPetroleum Processing and AnalysisFrench-language works237,207