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Record W2331943839 · doi:10.1021/jp107285r

In Situ High-Pressure Study of Sodium Amide by Raman and Infrared Spectroscopies

2010· article· en· W2331943839 on OpenAlexaff
Ang Liu, Yang Song

Bibliographic record

VenueThe Journal of Physical Chemistry B · 2010
Typearticle
Languageen
FieldMaterials Science
TopicHydrogen Storage and Materials
Canadian institutionsWestern University
Fundersnot available
KeywordsRaman spectroscopyOrthorhombic crystal systemInfraredChemistryInfrared spectroscopyAmbient pressureDiamond anvil cellAmideAnalytical Chemistry (journal)High pressureSodiumCrystal structureCrystallographyThermodynamicsOrganic chemistryOptics

Abstract

fetched live from OpenAlex

Here we report the first in situ high-pressure study of sodium amide (NaNH(2)) as an agent in potential hydrogen storage applications by using combined Raman and infrared (IR) spectroscopies at room temperature and pressures up to ~16 GPa. Starting with an orthorhombic crystal structure at ambient pressure, sodium amide was found to transform to two new phases upon compression as evidenced by the changes in the characteristic Raman and IR modes as well as by examining the pressure dependences of these modes. Raman and IR measurements on NaNH(2) collectively provided consistent information about the structural evolutions of NaNH(2) under compression. Upon decompression, all Raman and IR modes were completely recovered, indicating the reversibility of the pressure-induced transformations in the entire pressure region. The combined Raman and IR spectroscopic data together allowed for the analysis of possible structures of the new high-pressure phases of NaNH(2).

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.254

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.004
GPT teacher head0.240
Teacher spread0.236 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations32
Published2010
Admission routes1
Has abstractyes

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