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Record W2334233932 · doi:10.1021/cg401597p

Nanosized Nucleus-Supercooled Liquid Interfacial Free Energy and Thermophysical Properties of Early and Late Transition Liquid Metals

2014· article· en· W2334233932 on OpenAlexaff
Dong Hee Kang, Sangho Jeon, Hanbyeol Yoo, Takehiko Ishikawa, Junpei Okada, Paul‐François Paradis, Geun Woo Lee

Bibliographic record

VenueCrystal Growth & Design · 2014
Typearticle
Languageen
FieldMaterials Science
TopicMaterial Dynamics and Properties
Canadian institutionsInstitut National d'Optique
Fundersnot available
KeywordsSupercoolingNucleationThermodynamicsEnthalpy of fusionSurface energyMaterials scienceCrystal (programming language)Classical nucleation theoryEnthalpyChemical physicsMelting pointChemistry

Abstract

fetched live from OpenAlex

Crystal–liquid interfacial free energy is important to understand in crystal study, for example, nucleation, crystal growth, and vitrification. Here, we report the nanosized nucleus-supercooled liquid interfacial free energy of early and late transition liquid metals using the electrostatic levitation (ESL) technique and classical homogeneous nucleation theory (CNT). For the estimation of the interfacial free energy, we obtained thermophysical parameters of the transition liquid metals (Ti, Fe, Ni, Zr, Nb, Rh, and Hf), such as hypercooling limit (Δ T hyp ), specific heat ( C p ), total hemispherical emissivity (ε T ), and density (ρ). The estimated interfacial free energies of Ti, Ni, and Zr agreed well with a previous report having similar hypercooling limit and fusion enthalpy, while Fe, Nb, Rh, and Hf show different values from the report. This reflects the importance of accurate measurement of the two quantities. The obtained Turnbull’s coefficients (α) of the liquid metals is higher than 0.45. The interfacial free energy is discussed with configurationally different local order of the crystal and the liquid.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Theoretical or conceptual · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.003

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.015
GPT teacher head0.187
Teacher spread0.172 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designTheoretical or conceptual
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations38
Published2014
Admission routes1
Has abstractyes

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