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Record W2342400326 · doi:10.1177/026248931103000101

Development of Mechanically Stable Polymer-Based Silica Aerogel

2011· article· en· W2342400326 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueCellular Polymers · 2011
Typearticle
Languageen
FieldChemistry
TopicAerogels and thermal insulation
Canadian institutionsUniversity of Toronto
FundersNatural Sciences and Engineering Research Council of CanadaCanada Research Chairs
KeywordsAerogelMaterials sciencePolymerComposite materialDifferential scanning calorimetryThermogravimetric analysisSupercritical dryingScanning electron microscopeSpecific surface areaChemical engineeringOrganic chemistryChemistry

Abstract

fetched live from OpenAlex

Silica aerogels have attracted attention for many applications due to their unique properties such as low density (0.003 g/cm), mesoporosity (pore size 2–50 nm), high thermal insulation and high surface area (500–1200 m 2 /g). However, their fragility and environmental sensitivity restricts the use of monolithic silica aerogel. In this paper, silica aerogel that is crosslinked with diisocyanate is introduced and the effects of polymer concentration on aerogel properties, especially mechanical strength are discussed. Fracture of silica aerogel mainly occurs at the interface of secondary particles that are formed during aging. It is believed that if the surface of silica aerogel is covalently bonded to nanocast polymer coating, the interparticle necks become wider and can reinforce the structure of the aerogel. In this study, several characterizations are performed to investigate the properties of the aerogel. First, bulk density is measured to visualize the change in density with increase in crosslinker concentration. Brunauer Emmett and Teller (BET) illustrated the pore size, bulk density and surface area. The critical temperature up to which polymer crosslinked aerogel decompose was investigated by Thermogravimetric Analysis (TGA). The phase change in the aerogel was studied with Differential Scanning Calorimetry (DSC) testing. Using Scanning Electron Microscope (SEM), the nanoscale pore size and pore distribution throughout the aerogel surface were investigated. Furthermore, compression tests were performed to study the effect of crosslinking polymer on mechanical strength over non-crosslinked framework.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.035
Threshold uncertainty score0.994

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0070.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.034
GPT teacher head0.214
Teacher spread0.180 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it