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Record W2342685396 · doi:10.1002/cjce.22427

Production of synthetic fuels by high‐temperature co‐electrolysis of carbon dioxide and steam with Fischer‐Tropsch synthesis

2016· article· en· W2342685396 on OpenAlexvenueno aff
Lyman Frost, Elango Elangovan, Joseph Hartvigsen

Bibliographic record

VenueThe Canadian Journal of Chemical Engineering · 2016
Typearticle
Languageen
FieldEngineering
TopicChemical Looping and Thermochemical Processes
Canadian institutionsnot available
FundersOffice of Naval ResearchU.S. Air ForceNational Aeronautics and Space AdministrationU.S. Department of Energy
KeywordsNatural gasRenewable natural gasWaste managementSyngasCarbon dioxideCoalMethaneBiomass (ecology)Water gasRaw materialEnvironmental scienceChemistryFuel gasEngineeringHydrogenCombustion

Abstract

fetched live from OpenAlex

Numerous entities are currently involved in the production of synthetic fuels using various feedstock options including natural gas, refuse derived fuel, landfill gas, anaerobic digester gas, coal, and mixtures of these inputs. Current world‐class FT plants (∼15 900 m3/d or 100 000 barrels per day) require large deposits of natural gas (i.e. ∼1.78 m3/L/d or 10 MSCF/BPD means gas sources that can provide ∼10 billion m3 per year for plant lifetime). Modular Fischer‐Tropsch (FT) reactors currently under development have some unique features that reduce cost and provide the ability to utilize sources of natural gas, biomass, or other under‐utilized sources of energy that would otherwise not be developed. The current Ceramatec modular FT reactor operates with a fixed bed size of 10 cm diameter using an internal heat transfer structure to keep axial and radial temperature variation to < 10 °C. The internal heat transfer media avoids the traditional problem with fixed bed reactors of heat removal from highly exothermic reactions. These reactors can also be used to mitigate the current concern with emissions of carbon dioxide when used in conjunction with high‐temperature co‐electrolysis (HTCE) of carbon dioxide and water to produce synthesis gas and subsequently synthetic fuels. When combined with a non‐carbon source of electricity such as wind, solar, biomass gasification, or anaerobic digester gas, it is possible to store intermittent sources of electricity as liquid fuels for later use. The HTCE generally operates at a voltage of 1.32 V and a current density of ∼300 mA/cm2.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.005

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.002
GPT teacher head0.146
Teacher spread0.143 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations26
Published2016
Admission routes1
Has abstractyes

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