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Record W2407690456 · doi:10.1021/acssuschemeng.5b00796

Carbonized Lignin as Sustainable Filler in Biobased Poly(trimethylene terephthalate) Polymer for Injection Molding Applications

2015· article· en· W2407690456 on OpenAlexafffund
Petri Myllytie, Manjusri Misra, Amar K. Mohanty

Bibliographic record

VenueACS Sustainable Chemistry & Engineering · 2015
Typearticle
Languageen
FieldMaterials Science
TopicNatural Fiber Reinforced Composites
Canadian institutionsUniversity of GuelphDiscovery Centre
FundersNatural Sciences and Engineering Research Council of CanadaMinistero dello Sviluppo EconomicoOntario Ministry of Economic Development and Innovation
KeywordsMaterials scienceComposite materialFlexural strengthHeat deflection temperatureFiller (materials)Flexural modulusLigninPolymerThermoplasticCelluloseCarbonizationIzod impact strength testChemical engineeringOrganic chemistryUltimate tensile strengthChemistry

Abstract

fetched live from OpenAlex

High Resolution Image Download MS PowerPoint Slide Light weight and sustainability are the key drivers in the development of novel biobased thermoplastic compounds for automotive applications. This paper reports the engineering properties of thermoplastic compound consisting of a novel bioresourced carbon filler in combination with partially biobased poly(trimethylene terephthalate). The bioresourced carbon filler, which was derived from lignin residue of cellulosic ethanol production, has a clear advantage in terms of density compared to glass fiber and other minerals, and shows potential for weight reduction with 7% lower density at 20% filler content. Polymer processing conditions were optimized in terms of thermomechanical properties, and use of a reactive chain extender additive was studied for improving the performance of the compound. At the optimized conditions, good dimensional stability, 89% increase in heat deflection temperature, 60% increase in flexural modulus, and 14% increase in flexural strength was attained in comparison to neat PTT polymer. Theoretical modeling based on a rule-of-mixture approach showed good agreement of the predicted and experimental modulus of the studied composites. When compared to existing mineral filled engineering polyester resin, many properties of the prepared compounds were on a comparable or favorable level, indicating good potential of the bioresourced carbon filler for light weighting and highly sustainable engineering applications.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.015
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.001
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.007
GPT teacher head0.232
Teacher spread0.225 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations45
Published2015
Admission routes2
Has abstractyes

Explore more

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