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Record W2471713401 · doi:10.1002/slct.201600713

Highly Ordered Rectangular Columnar Ionic Liquid Crystals: A More Efficient Medium for Intramolecular Diels Alder Reactions

2016· article· en· W2471713401 on OpenAlexafffund
Dat Tien, Andreea R. Schmitzer

Bibliographic record

VenueChemistrySelect · 2016
Typearticle
Languageen
FieldChemical Engineering
TopicIonic liquids properties and applications
Canadian institutionsUniversité de Montréal
FundersUniversité de MontréalCentre in Green Chemistry and Catalysis
KeywordsIntramolecular forceIonic liquidDiels–Alder reactionYield (engineering)SolventIonic bondingLiquid crystalSelectivityMaterials sciencePhase (matter)BenzeneCrystal (programming language)ChemistryOrganic chemistryPhotochemistryIonCatalysisComposite material

Abstract

fetched live from OpenAlex

Abstract Herein, we present the synthesis, the thermal and mesophormic properties of trialkyl(1,3,5‐benzene)trisimidazolium salts. These salts form highly ordered rectangular columnar ionic liquid crystal phases and can be used as reaction media for Diels Alder reactions. The use of the ionic liquid crystal phase favours the formation of the intramolecular Diels Alder products, even in high concentration reaction conditions. We show that the ionic liquid crystal phase can be recycled and reused as solvent for at least 10 times, without any loss of yield or selectivity in the Diels Alder reaction.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.149
Threshold uncertainty score0.816

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.010
GPT teacher head0.236
Teacher spread0.226 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations11
Published2016
Admission routes2
Has abstractyes

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