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Record W2478870599 · doi:10.1021/cm0351240

Nanostructured Lanthanide-Doped Lu<sub>2</sub>O<sub>3</sub> Obtained by Propellant Synthesis

2004· article· en· W2478870599 on OpenAlexaff
Stefano Polizzi, S. Bucella, Adolfo Speghini, Fiorenzo Vetrone, Rafik Naccache, J. Christopher Boyer, John A. Capobianco

Bibliographic record

VenueChemistry of Materials · 2004
Typearticle
Languageen
FieldMaterials Science
TopicLuminescence Properties of Advanced Materials
Canadian institutionsConcordia University
Fundersnot available
KeywordsIonic radiusLanthanideMaterials scienceNanocrystalline materialLuminescenceDopingAnalytical Chemistry (journal)CeriumIonNanotechnologyChemistryMetallurgy

Abstract

fetched live from OpenAlex

Lu 1.98 Ln 0.02 O 3 (Ln = Nd, Eu, and Er) powders obtained by propellant synthesis were characterized using XRD, SAXS, TEM, and SEM. Samples have a very porous, open morphology with fractal scaling properties. The building blocks of the fractal aggregates are 60−90 nm lanthanide-doped cubic Lu 2 O 3 crystalline particles, which exhibit changes in the lattice parameter proportional to the lanthanide ionic radius. The NIR luminescence spectrum of nanocrystalline Lu 2 O 3:Nd 3+ was measured and emission was observed from the 4 F 3/2 excited state to the 4 I J (9/2, 11/2, 13/2, 15/2) state. The spectral features are very similar to those of a bulk material of identical composition prepared for comparison, though with a noticeable difference in the relative intensity of the 4 F 3/2 → 4 I 9/2 and 4 F 3/2 → 4 I 11/2 transitions. The spectroscopic-quality parameter ( X ) for nanocrystalline samples was calculated and was found to be higher than for the bulk.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.001
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.002
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.001
Meta-epidemiology (narrow)0.0010.001
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.000
Science and technology studies0.0000.001
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.007
GPT teacher head0.201
Teacher spread0.193 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations48
Published2004
Admission routes1
Has abstractyes

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