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Record W2523367608 · doi:10.1021/cm071244m

Synthesis and Characterization of Carbon-Doped TiO<sub>2</sub> Nanostructures with Enhanced Visible Light Response

2007· article· en· W2523367608 on OpenAlexaff
Guosheng Wu, Tomohiro Nishikawa, Bunsho Ohtani, Aicheng Chen

Bibliographic record

VenueChemistry of Materials · 2007
Typearticle
Languageen
FieldEnergy
TopicTiO2 Photocatalysis and Solar Cells
Canadian institutionsLakehead University
Fundersnot available
KeywordsMaterials scienceAnataseCarbon fibersCarbon nanotubePhotocurrentDopingInert gasNanotechnologyChemical engineeringBand gapChemical vapor depositionArgonPhotocatalysisOptoelectronicsChemistryOrganic chemistryComposite material

Abstract

fetched live from OpenAlex

Carbon-doped TiO 2 micro-/nanospheres and nanotubes have been synthesized via a single source chemical vapor deposition in an inert atmosphere. Organic compound Ti(OC 4 H 9 ) 4 was used as the titanium, oxygen, and carbon source, while argon served as the carrier gas. The effect of the temperature, substrate, and the flow rate of the carrier gas is investigated. The diameter of the formed carbon-doped TiO 2 spheres can be adjusted from 100 nm to several micrometers by varying the flow rate of the carrier gas. The as-prepared TiO 2 nanotubes are highly ordered with a diameter of about 100 nm and a wall thickness of around 15 nm. The estimated optical band gap is 2.78 eV for the formed carbon-doped TiO 2 microspheres and 2.72 eV for the synthesized carbon-doped TiO 2 nanotubes, both of which are much smaller than that of bulk anatase TiO 2 (3.20 eV). The photocurrent of the carbon-doped TiO 2 spheres is much higher than that of commercial P-25, which is currently considered as one of the best TiO 2 photocatalysts, especially under visible light irradiation. The possible mechanism of the formation of TiO 2 spheres and nanotubes is also discussed.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.002

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0010.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.004
GPT teacher head0.193
Teacher spread0.189 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations279
Published2007
Admission routes1
Has abstractyes

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