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Record W2551201640 · doi:10.1002/aenm.201601602

Amorphous MoS<sub>3</sub> Infiltrated with Carbon Nanotubes as an Advanced Anode Material of Sodium‐Ion Batteries with Large Gravimetric, Areal, and Volumetric Capacities

2016· article· en· W2551201640 on OpenAlexafffund
Hualin Ye, Lu Wang, Shuo Deng, Xiaoqiao Zeng, Kaiqi Nie, Paul N. Duchesne, Bo Wang, Simon Liu, Junhua Zhou, Feipeng Zhao, Na Han, Peng Zhang, Jun Zhong, Xuhui Sun, Youyong Li, Yanguang Li, Jun Lü

Bibliographic record

VenueAdvanced Energy Materials · 2016
Typearticle
Languageen
FieldEngineering
TopicAdvancements in Battery Materials
Canadian institutionsUniversity of WaterlooDalhousie University
FundersNatural Sciences and Engineering Research Council of CanadaNational Natural Science Foundation of ChinaU.S. Department of Energy
KeywordsMaterials scienceAnodeGravimetric analysisAmorphous solidChemical engineeringElectrodeAmorphous carbonCarbon nanotubeCathodeIonPrecipitationAdsorptionNanotechnologyOrganic chemistry

Abstract

fetched live from OpenAlex

The search for earth‐abundant and high‐performance electrode materials for sodium‐ion batteries represents an important challenge to current battery research. 2D transition metal dichalcogenides, particularly MoS 2 , have attracted increasing attention recently, but few of them so far have been able to meet expectations. In this study, it is demonstrated that another phase of molybdenum sulfide—amorphous chain‐like MoS 3 —can be a better choice as the anode material of sodium‐ion batteries. Highly compact MoS 3 particles infiltrated with carbon nanotubes are prepared via the facile acid precipitation method in ethylene glycol. Compared to crystalline MoS 2 , the resultant amorphous MoS 3 not only exhibits impressive gravimetric performance—featuring excellent specific capacity (≈615 mA h g −1 ), rate capability (235 mA h g −1 at 20 A g −1 ), and cycling stability but also shows exceptional volumetric capacity of ≈1000 mA h cm −3 and an areal capacity of &gt;6.0 mA h cm −2 at very high areal loadings of active materials (up to 12 mg cm −2 ). The experimental results are supported by density functional theory simulations showing that the 1D chains of MoS 3 can facilitate the adsorption and diffusion of Na + ions. At last, it is demonstrated that the MoS 3 anode can be paired with an Na 3 V 2 (PO 4 ) 3 cathode to afford full cells with great capacity and cycling performance.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.003
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0010.001
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0010.001
Science and technology studies0.0000.000
Scholarly communication0.0000.001
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.005
GPT teacher head0.190
Teacher spread0.185 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations195
Published2016
Admission routes2
Has abstractyes

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