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Record W2558125322 · doi:10.1107/s2053273314082904

Tetrakis(μ-2-phenylacetato-κ2O:O′) bis{(DMSO κO′)]copper(II)}(Cu-Cu)]

2014· article· en· W2558125322 on OpenAlexaff
Meriem Benslimane, Yasmine K. Redjel, Georges Dénès, Hocine Mérazig

Bibliographic record

VenueActa Crystallographica Section A Foundations and Advances · 2014
Typearticle
Languageen
FieldMedicine
TopicMetal complexes synthesis and properties
Canadian institutionsConcordia University
Fundersnot available
KeywordsChemistryCarboxylatePhenylacetateCopperCobaltTransition metalCrystallographyOctahedronCrystal structureDivalentStereochemistryMedicinal chemistryInorganic chemistryOrganic chemistry

Abstract

fetched live from OpenAlex

Carboxylate groups may interact as bridging ligands with divalent transition metals present in biological environments, thereby altering the bioavailability of drugs. Moreover, it is well known that many complexes of divalent transition metals are capable of catalyzing the hydrolysis of RNA (Stem et al., 1990; Kimura, 1994). The coordination chemistry of Cu2+ complexes bridged by phenylacetate has been reported. We have found only two reports of a dinuclear Co2+ complexes, namely tetrakis (phenylacetato)bis[(quinoline-N)-cobalt(II)](Cui et al.,1999),μ-aqua-κ2O:O-di-μ-phenylacetato-κ4O:O′-bis[(1,10-phenanthroline-κ2N,N′) (phenyl acetato-κO)cobalt(II)](Kong et al., 2005) and dinuclear Cu2+ complex, namely tetrakis (phenylacetato)bis-[(N,N-dimethylformamide)copper(II)], in which all phenylacetate groups are in bidendate bridging modes. In this presentation, the crystal structure of a new dimeric complex obtained by reaction of phenylacetic acid with copper(II) acetate is described. Each Cu(II) atom is six-coordinated by five O atoms from carboxylate groups of the phenylacetate and DMSO ligands and is completed by a Cu-Cu bond in a strongly distorted octahedral coordination, in which an inversion center is located at the mid-point of the Cu-Cu bond with a Cu...Cu distance of 2.6321(4) Å. This is longer than the 2.251(2)Å distance found in the polymeric complex [Cu2(C8H7O2)4]n. However, it is similar to the 2.6414(8) Å and 2.6261(8)Å distances found in the complex [Cu2(C8H7O2)4(C3H7NO)2] (Kong et al., 2005). The Cu-O phenylacetate bond length lies in the range 1.9644(14) to 1.9734 (14) Å and the Cu-ODMSO bond length is 2.1319(13) Å.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Not applicable · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.975
Threshold uncertainty score0.949

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0010.000
Scholarly communication0.0000.001
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.023
GPT teacher head0.273
Teacher spread0.250 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designNot applicable
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2014
Admission routes1
Has abstractyes

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