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Record W2558804214 · doi:10.1107/s2053273314089104

Connectivity and formula-generating functions for sheet-silicate minerals

2014· article· en· W2558804214 on OpenAlexaff
F. C. Hawthorne

Bibliographic record

VenueActa Crystallographica Section A Foundations and Advances · 2014
Typearticle
Languageen
FieldEarth and Planetary Sciences
TopicBuilding materials and conservation
Canadian institutionsUniversity of Manitoba
Fundersnot available
KeywordsTetrahedronNet (polyhedron)CombinatoricsSimple (philosophy)Plane (geometry)StoichiometryTopology (electrical circuits)MathematicsCrystallographyGeometryChemistry

Abstract

fetched live from OpenAlex

Silicate sheets may be described by two-dimensional nets in which the vertices of the net are occupied by tetrahedra, and the edges of the net represent linkages between tetrahedra. A plane net must contain 3-connected vertices, but not all vertices need to be 3-connected. Simple silicate structures may thus be generated from simple 3-connected plane nets (e.g. 6 3 , 4.8 2 , 4.6.8, (4.6.8) 2 (6.8 2 ) 1 , etc.). More complicated silicate nets may be generated by various "building operations": (1) Insertion: insertion of 2- and 4-connected vertices into 3-connected plane nets; (2) Repetition: generation of double (or triple) nets by topological symmetry operations that retain transitivity at the junction between the repeated elements. Diversity is also introduced within the sheets of tetrahedra by [1] adjacent apical tetrahedron vertices pointing in the same or different directions, and [2] by folding of the sheets. For simple structures, net type strongly affects the stoichiometry of the resultant structure as the unit cells of the various nets are of different sizes (and shapes), although the stoichiometry may also be affected by non-tetrahedral components. Building operations strongly affect the stoichiometry of the resultant sheet, and this effect may be quantified. We define a formula-generating function F(k,l,...) that generates the formula of a sheet with specific topological features denoted by the indices k,l,... . A simple 3-connected net results in sheets of the form (T 2 O 5 )n where n denotes the number of (T 2 O 5 )n in the unit cell of the underlying net (for 6 3 , n = 1; for 4.8 2 , n = 2; for (4.6.8) 2 (6.8 2 ) 1 , n = 3, etc). Plane nets with k 3-connected vertices and l inserted 2-connected vertices result in sheets of the form [T(k+l) O(2.5k+3l)], where (...) are subscripted. Single- and double-sheet structures may be generated from the function F(k,l) = T(N{k+l}) O(N{3k+2.5l}-n{N-1}) where N = 1 and 2 for single- and double-sheets, respectively, and (...) are subscripted.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Observational · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.572
Threshold uncertainty score0.636

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0010.000
Scholarly communication0.0000.001
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.014
GPT teacher head0.229
Teacher spread0.215 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designObservational
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2014
Admission routes1
Has abstractyes

Explore more

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