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3D Conformal Modification of Electrospun Silk Nanofibers with Nanoscaled ZnO Deposition for Enhanced Photocatalytic Activity

2016· article· en· W2562953749 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueACS Biomaterials Science & Engineering · 2016
Typearticle
Languageen
FieldMaterials Science
TopicSilk-based biomaterials and applications
Canadian institutionsSimon Fraser University
FundersMinistry of Science and Technology of the People's Republic of ChinaMinistry of Education of the People's Republic of ChinaNational Natural Science Foundation of China
KeywordsMaterials sciencePhotocatalysisWurtzite crystal structureAtomic layer depositionNanotechnologyOxideNanofiberElectrospinningPhotodegradationChemical vapor depositionSILKDeposition (geology)NanomaterialsMetalLayer (electronics)Chemical engineeringZincComposite materialMetallurgyPolymerCatalysisOrganic chemistry

Abstract

fetched live from OpenAlex

Nanostructured metal oxide materials have drawn great attention because of their enhanced semiconducting, electrical, optical, sensing, and chemical catalyzing properties. The application of metal oxides in biomedicine has recently emerged as a promising field, especially in the format of organic/metal oxide composites. However, the existing methods for fabricating organic/metal oxide materials revealed limitations on the precise control over the deposition of metal oxides and the maintenance of organic nanostructures. Here, we developed an approach for the fabrication of composite materials by depositing metal oxides on the nanostructured organic templates through atomic layer deposition (ALD). With this method, we fabricated a series of silk fibroin/ZnO composites at varied deposition temperatures. The results demonstrated that the ZnO layer had a 3D conformality and hexagonal wurtzite structure, and the deposition thickness was well controlled. The photocatalytic activity of silk/ZnO composites was confirmed by the photodegradation of Rh-B under UV exposure, and the efficiency was found to be temperature dependent. These results demonstrated the successful integration of organic materials with metal oxides through an easy and controllable approach for the development of multifunctional organic/metal oxide biomaterials.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.148
Threshold uncertainty score0.749

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.001
Open science0.0010.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.010
GPT teacher head0.237
Teacher spread0.228 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it