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Record W2581414942 · doi:10.1021/acs.iecr.6b04412

A Kinetic Uptake Study of Roxarsone Using Cross-Linked Chitosan Beads

2017· article· en· W2581414942 on OpenAlexafffund
Mohammad H. Mahaninia, Lee D. Wilson

Bibliographic record

VenueIndustrial & Engineering Chemistry Research · 2017
Typearticle
Languageen
FieldEnvironmental Science
TopicAdsorption and biosorption for pollutant removal
Canadian institutionsUniversity of Saskatchewan
FundersUniversity of Saskatchewan
KeywordsChitosanGlutaraldehydeEpichlorohydrinAdsorptionSorbentBeadChemistryChromatographyScanning electron microscopePacked bedChemical engineeringAnalytical Chemistry (journal)Materials scienceNuclear chemistryPolymer chemistryOrganic chemistryComposite material

Abstract

fetched live from OpenAlex

The adsorptive behavior of chitosan bead materials with roxarsone (ROX) was studied using a fixed bed column and a one-pot setup to evaluate the kinetic and thermodynamic adsorption parameters. The role of variable surface chemical properties of chitosan beads on the adsorption properties with ROX was investigated using a dye-based method, contact angle measurements, powder X-ray diffraction, scanning electron microscopy, and atomic force microscopy. The equilibrium uptake ( q e; mg ROX/g sorbent) values are listed in ascending order: non-cross-linked chitosan bead (52.5 mg/g) < chitosan bead cross-linked with epichlorohydrin (89.1 mg/g) < chitosan bead cross-linked with glutaraldehyde (104 mg/g). The results agree with uptake values obtained using a fixed bed column, where cross-linked chitosan beads display relatively rapid ROX uptake (0.121 min –1 ) relative to that of the non-cross-linked chitosan bead (0.053 min –1 ). These observed trends can be understood according to the hydrophile–lipophile balance and pore structure properties of cross-linked chitosan beads. The column bed removal efficiency (65.2%) increased for chitosan beads cross-linked with glutaraldehyde as the packed bed adsorbent material.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.011
Threshold uncertainty score0.022

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0010.001
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0010.001
Open science0.0000.000
Research integrity0.0010.001
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.168
GPT teacher head0.388
Teacher spread0.220 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations33
Published2017
Admission routes2
Has abstractyes

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