MétaCan
Menu
Back to cohort
Record W2584382404 · doi:10.1021/jacs.6b12814

The Power of Packing: Metallization of an Organic Semiconductor

2017· article· en· W2584382404 on OpenAlexafffund
Aaron Mailman, Alicea A. Leitch, Wenjun Yong, Eden Steven, Stephen M. Winter, Robert C. M. Claridge, Abdeljalil Assoud, John S. Tse, Serge Desgreniers, Richard A. Secco, Richard T. Oakley

Bibliographic record

VenueJournal of the American Chemical Society · 2017
Typearticle
Languageen
FieldEngineering
TopicOrganic Electronics and Photovoltaics
Canadian institutionsUniversity of OttawaUniversity of SaskatchewanWestern UniversityUniversity of Waterloo
FundersCanada Foundation for InnovationNatural Sciences and Engineering Research Council of CanadaDivision of Materials ResearchCanada Research ChairsGovernment of CanadaNational Science Foundation
KeywordsChemistrySemiconductorOrganic semiconductorPower (physics)NanotechnologyEngineering physicsOptoelectronicsOrganic chemistryThermodynamics

Abstract

fetched live from OpenAlex

Benzoquino-bis-1,2,3-dithiazole 5 is a closed shell, antiaromatic 16π-electron zwitterion with a small HOMO–LUMO gap. Its crystal structure consists of planar ribbon-like molecular arrays packed into offset layers to generate a “brick-wall” motif with strong 2D interlayer electronic interactions. The spread of the valence and conduction bands, coupled with the narrow HOMO–LUMO gap, affords a small band gap semiconductor with σ RT = 1 × 10 –3 S cm –1 and E act = 0.14 eV for transport within the brick-wall arrays. Closure of the band gap to form an all-organic molecular metal with σ RT > 10 1 S cm –1 can be achieved by the application of pressure to 8 GPa.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.178

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.008
GPT teacher head0.232
Teacher spread0.224 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations58
Published2017
Admission routes2
Has abstractyes

Explore more

Same venueJournal of the American Chemical SocietySame topicOrganic Electronics and PhotovoltaicsFrench-language works237,207