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Record W2586088456 · doi:10.1002/cjce.22808

Individual and interaction effects of operating parameters on the photocatalytic degradation under visible light illumination: Response surface methodological approach

2017· article· en· W2586088456 on OpenAlexaffvenue
Mehrzad Feilizadeh, Mohammad Rahimi, S. Mohammad Esmaeil Zakeri, Nader Mahinpey, Manouchehr Vossoughi, Mojtaba Qanbarzadeh

Bibliographic record

VenueThe Canadian Journal of Chemical Engineering · 2017
Typearticle
Languageen
FieldEnergy
TopicAdvanced Photocatalysis Techniques
Canadian institutionsUniversity of Calgary
Fundersnot available
KeywordsResponse surface methodologyPhotocatalysisDegradation (telecommunications)Visible spectrumMaterials scienceReagentPollutantChemical engineeringAnalytical Chemistry (journal)ChemistryChromatographyCatalysisComputer scienceOptoelectronicsOrganic chemistry

Abstract

fetched live from OpenAlex

ABSTRACT In this study, for the first time a statistical analysis based on the response surface methodology (RSM) was employed to investigate individual and interaction effects of key operating parameters of the photocatalytic degradation under visible‐light irradiation using Ag‐S/PEG/TiO 2 . Ag‐S/PEG/TiO 2 is a visible‐light‐driven photocatalyst and was synthesized (based on earlier research) by co‐doping of TiO 2 with silver and sulphur and addition of polyethylene glycol (as a reagent template). In addition, the model pollutant was methylene orange (MO) and the studied operating parameters included the photocatalyst loading, initial concentration of the pollutant, and pH of the solution. The statistics‐based experimental design and RSM was utilized to find a quadratic model as a functional relationship between the degradation efficiency and the three operating parameters. The regression analysis with R 2 value of 0.9678 showed a close fit between the model prediction and experimental data of the degradation efficiency. The analysis of variance based on the model indicated that pH of the solution was the most influential factor, while the two other operating parameters were also significant. The efficiency of MO degradation reached 94.0 % under the optimum conditions (i.e. photocatalyst loading of 1.20 g/L, MO concentration of 5 mg/L, and pH of 2).

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.003
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.061
Threshold uncertainty score0.368

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.003
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.050
GPT teacher head0.291
Teacher spread0.242 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations34
Published2017
Admission routes2
Has abstractyes

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