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Record W2588205154 · doi:10.1002/cjce.22813

Adsorption of copper on glass beads coated with chitosan: Stirred batch and fixed bed analysis

2017· article· en· W2588205154 on OpenAlexvenueno aff
Marlon de Souza Gama, F. Murilo T. Luna, Juliana Q. Albarelli, Marisa Masumi Beppu, Rodrigo Silveira Vieira

Bibliographic record

VenueThe Canadian Journal of Chemical Engineering · 2017
Typearticle
Languageen
FieldEnvironmental Science
TopicAdsorption and biosorption for pollutant removal
Canadian institutionsnot available
FundersConselho Nacional de Desenvolvimento Científico e TecnológicoFundação de Amparo à Pesquisa do Estado de São Paulo
KeywordsAdsorptionChitosanMass transferCopperDiffusionMaterials scienceMass transfer coefficientChemical engineeringSurface diffusionInertComposite materialChromatographyChemistryThermodynamicsMetallurgyOrganic chemistry

Abstract

fetched live from OpenAlex

Chitosan is a natural polymer largely studied for heavy metal adsorption applications, since the amino and hydroxyl groups present in its structure can act as chelation sites. However, this material presents some drawbacks as an adsorbent due to its low mechanical strength. Studies have shown that the use of immobilized chitosan on glass beads can improve the mechanical strength of adsorbent and enhance mass transfer properties. For this reason, stirred batch experiments of copper adsorption on chitosan immobilized onto glass beads were performed to estimate the surface diffusion coefficient and the chitosan film thickness, considering an inert solid glass core. The kinetic data were modelled by a surface diffusion model incorporating the external film mass transfer resistance. Column experiments were also performed for copper solution at different flow rates and a film‐surface diffusion model was used to describe the breakthrough adsorption experiments, using the chitosan film thickness estimated from the batch experiment (φ = 2.5 µm). The input parameters for this model were determined by batch experiments or estimated from correlations available in the open literature. The surface diffusion coefficients (0.98–1.72 × 10−10 cm2 · min−1) of copper in the chitosan film for different flow rates were estimated. The experimental data and the model agreed, indicating that the film thickness and the mass transfer parameters were well predicted.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.044
Threshold uncertainty score0.087

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0010.001
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0010.001
Bibliometrics0.0010.002
Science and technology studies0.0010.000
Scholarly communication0.0010.000
Open science0.0010.000
Research integrity0.0010.001
Insufficient payload (model declined to judge)0.0010.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.008
GPT teacher head0.195
Teacher spread0.187 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations7
Published2017
Admission routes1
Has abstractyes

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Same venueThe Canadian Journal of Chemical EngineeringSame topicAdsorption and biosorption for pollutant removalFrench-language works237,207