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Record W2594959252 · doi:10.3390/met7030097

Impact of the Solidification Rate on the Chemical Composition of Frozen Cryolite Bath

2017· article· en· W2594959252 on OpenAlexafffund
Sándor Poncsák, László I. Kiss, Sébastien Guérard, Jean‐François Bilodeau

Bibliographic record

VenueMetals · 2017
Typearticle
Languageen
FieldChemical Engineering
TopicMolten salt chemistry and electrochemical processes
Canadian institutionsRio Tinto (Canada)Université du Québec à Chicoutimi
FundersNatural Sciences and Engineering Research Council of CanadaUniversité du Québec à Chicoutimi
KeywordsCryoliteDiffractometerScanning electron microscopeChemical compositionMaterials scienceAnalytical Chemistry (journal)Thermal conductivityRecrystallization (geology)MineralogyChemistryMetallurgyAluminiumComposite materialChromatography

Abstract

fetched live from OpenAlex

Solidification of cryolite (Na3AlF6)-based bath takes place at different rates along the sideledge, and around alumina rafts and new anodes. The solidification rate has a significant impact on the structure and the chemical composition that determine the thermal conductivity and thus the thickness of sideledge, or the duration of the existence of the temporary frozen bath layers in other cases. Unfortunately, samples that can be collected in industrial cells are formed under unknown, spatially and temporally varying conditions. For this reason, frozen bath samples were created under different heat flux conditions in a well-controlled laboratory environment using the so-called cold finger technique. The samples were analyzed by X-ray Diffractometer (XRD) and Scanning Electron Microscope (SEM) in Back Scattering (BS) mode in order to obtain spatial distribution of chemical composition. Results were correlated with structural analysis. XRD confirmed our earlier hypothesis of recrystallization of cryolite to chiolite under medium heat flux regime. Lower α-alumina, and higher γ-alumina content in the samples obtained with very high heating rate suggest that fast cooling reduces α–γ conversion. In accordance with the expectation, SEM-BS revealed significant variation of the Na/Al ratio in the transient sample.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.004
Threshold uncertainty score0.251

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.024
GPT teacher head0.286
Teacher spread0.262 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations8
Published2017
Admission routes2
Has abstractyes

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