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Record W2598747157 · doi:10.2118/184575-ms

Analysis and Optimization of H2S Scavenger Systems Using X-Ray Fluorescence Spectroscopy

2017· article· en· W2598747157 on OpenAlexaboutno aff
Dave Horton, Derrick Bakuska, Jeff Soderberg

Bibliographic record

VenueSPE International Conference on Oilfield Chemistry · 2017
Typearticle
Languageen
FieldEngineering
TopicIndustrial Gas Emission Control
Canadian institutionsnot available
Fundersnot available
KeywordsSulfurScavengerChemistryMatrix (chemical analysis)Hydrogen sulfideDetection limitAnalytical Chemistry (journal)Environmental chemistryChromatographyRadicalOrganic chemistry

Abstract

fetched live from OpenAlex

Abstract Field methods are available for the determination of dithiazine content in spent hydrogen sulfide scavengers. While these methods are useful, accuracy of the assay and interference from other chemical species or matrix effects can limit the utility of these methodologies. Due to the limitations of these methods, alternate analytical techniques were investigated. An analytical method has been developed using x-ray fluorescent (XRF) techniques that rapidly provides accurate results for total sulfur content in these scavengers. The method uses analytical equipment commercially available for sulfur in oil analysis. Sulfur compound speciation is not possible with XRF techniques, however speciation is not a critical factor in optimization as the goal is to maximize sulfur uptake while limiting dithiazine content and available sulfur to form dithiazine. The method finds application in any other scavenger solutions where soluble sulfur species are present, for example, alkanolamines or solvent based such as polyethylene glycol methyl esters. Instrument calibration is dependent upon the matrix being analyzed; however the method is robust within similar matrices of material. Instruments used for this application are light, portable and easy to use in a laboratory environment or a field environment. The method has been applied in a variety of locations in the United States and Canada to aid in optimization of scavenger application. Verification of the accuracy of the method was confirmed by random sampling and combustion analysis of the random sample of spent scavenger at Alberta Sulphur Research.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Simulation or modeling · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.436
Threshold uncertainty score0.823

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.032
GPT teacher head0.279
Teacher spread0.247 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designSimulation or modeling
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations1
Published2017
Admission routes1
Has abstractyes

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