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Record W2605014117 · doi:10.1021/acs.chemmater.6b05356

γ-Fe<sub>2</sub>O<sub>3</sub>@CNTs Anode Materials for Lithium Ion Batteries Investigated by Electron Energy Loss Spectroscopy

2017· article· en· W2605014117 on OpenAlexaff
Xiaoxin Lv, Jiujun Deng, Biqiong Wang, Jun Zhong, Tsun‐Kong Sham, Xuhui Sun, Xueliang Sun

Bibliographic record

VenueChemistry of Materials · 2017
Typearticle
Languageen
FieldEngineering
TopicAdvancements in Battery Materials
Canadian institutionsWestern University
FundersPriority Academic Program Development of Jiangsu Higher Education InstitutionsGovernment of Jiangsu ProvinceNational Natural Science Foundation of China
KeywordsAnodeMaterials scienceLithium (medication)Carbon nanotubeChemical engineeringCapacity lossMaghemiteEnergy storageElectron energy loss spectroscopyComposite numberIonElectrodeSpectroscopyCurrent densityNanotechnologyNanoparticleComposite materialTransmission electron microscopyChemistry

Abstract

fetched live from OpenAlex

Atomic layer deposition was employed to deposit maghemite (γ-Fe 2 O 3 ) nanoparticles on carbon nanotubes (CNTs) to prepare the γ-Fe 2 O 3 @CNTs composites, which exhibit a superior lithium storage performance as the anode of lithium ion batteries (LIBs). The high reversible capacity of 859.7 mA h/g was observed after 400 cycles at a current density of 500 mA/g. Even at the high current density of 10000 mA/g, the specific cyclic capacity of 464.4 mA h/g can still be obtained. Furthermore, electron energy loss spectroscopy results reveal that the Fe chemical state plays a critical role in the evolution of the capacity of γ-Fe 2 O 3 @CNTs composite anodes during the cycling process. The incomplete conversion of the chemical state in γ-Fe 2 O 3 reduces the capacity, while the recovery of the chemical state of γ-Fe 2 O 3 during the cycling process may cause the increase in capacity. This work provides insight into understanding the detailed working mechanism of transition metal oxides in LIBs, which helps in the design of electrode materials with promising lithium storage performance.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.010
Threshold uncertainty score0.999

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0010.001
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0010.001
Open science0.0010.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.009
GPT teacher head0.229
Teacher spread0.220 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations83
Published2017
Admission routes1
Has abstractyes

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