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Record W2615373355 · doi:10.1088/2053-1591/aa742d

Zr-doped TiO<sub>2</sub>nanoparticles synthesized via a sol–gel route and their application in dye-sensitized solar cells for thermo-stabilization

2017· article· en· W2615373355 on OpenAlexafffund
Anastasia Pasche, Bernd Grohe, Silvia Mittler, Paul A. Charpentier

Bibliographic record

VenueMaterials Research Express · 2017
Typearticle
Languageen
FieldEnergy
TopicTiO2 Photocatalysis and Solar Cells
Canadian institutionsWestern University
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsDye-sensitized solar cellMaterials scienceAnataseCrystallinityChemical engineeringDopingCalcinationRutileThermal stabilityNanotechnologySol-gelPhotovoltaic systemFabricationSolar cellSpecific surface areaNanoparticlePhotocatalysisOptoelectronicsComposite materialCatalysisOrganic chemistryChemistryElectrode

Abstract

fetched live from OpenAlex

Dye-sensitized solar cells (DSSCs) are regarded as one of the most promising solar cells amongst third-generation photovoltaic technologies, particularly due to their low cost, easy preparation, and minor environmental impact compared to earlier-generation devices. However, they have been challenged by thermal energy losses and low cell efficiencies. This work examined the incorporation of zirconium (Zr) into the crystal lattice of titania nanoparticles (nTiO 2 ) for subsequent fabrication into the photo anode of the DSSCs. The results showed that Zr doping of nTiO 2 inhibited the anatase-rutile phase transition. Higher calcination temperatures gave increased titania crystallinity, and stabilized the nTiO 2 aggregate pore structure and specific surface area, consequently improving the DSSC device performance. A doping concentration of 5 mol % Zr into the nTiO 2 demonstrated the best resistance against thermal degradation, achieving an optimized retention of specific surface area. Solar simulation confirmed the results, indicating better heat stability, although lowering the DSSC efficiencies.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.002

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.038
GPT teacher head0.298
Teacher spread0.260 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations13
Published2017
Admission routes2
Has abstractyes

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