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Record W2621088979 · doi:10.1002/cjce.22906

The effect of inorganic solids on emulsion layer growth in asphaltene‐stabilized water‐in‐oil emulsions

2017· article· en· W2621088979 on OpenAlexafffundvenue
Michaela K. McGurn, Elaine N. Baydak, Danuta M. Sztukowski, Harvey W. Yarranton

Bibliographic record

VenueThe Canadian Journal of Chemical Engineering · 2017
Typearticle
Languageen
FieldEngineering
TopicEnhanced Oil Recovery Techniques
Canadian institutionsShell (Canada)University of Calgary
FundersNatural Sciences and Engineering Research Council of CanadaCanada Research ChairsShell CanadaSuncor Energy Incorporated
KeywordsEmulsionAsphalteneChemical engineeringMaterials scienceLayer (electronics)Composite materialEngineering

Abstract

fetched live from OpenAlex

Oilfield emulsions are often stabilized by asphaltenes but inorganic solids can impact both emulsion stability and rag layer accumulation. In this study, the effect of inorganic solids on emulsion stability and emulsion layer growth was investigated using batch and continuous separations performed on water‐in‐oil emulsions stabilized by asphaltenes. The emulsions were prepared at 60 °C from an organic phase consisting of solids, asphaltenes, n‐heptane, and toluene and an initial water phase volume of 0.50. Three types of coarse solids were considered: 12 μm kaolin, 18–32 μm silica, and 32–63 μm silica with wettabilities ranging from 50 to 125°. In batch experiments, the coalescence rate was determined from the change in height of the free water and oil layers over time as the emulsion coalesced. In continuous experiments, emulsion layer growth was measured as the emulsion was continuously fed into a vertical separator. The data were modelled with a material balance that included a coalescence rate equation. In the absence of solids, the continuous emulsion layer growth rate and ultimate stability correlated well to batch coalescence parameters. The addition of the coarse solids at concentrations below 5 g/L accelerated coalescence rates. Above 5 g/L, the solids increased emulsion stability indicating that they form a steric barrier between the droplets. Even if the feed is below this threshold, the solids accumulate in the rag layer until the threshold is reached, the emulsion becomes stable, and the performance of the continuous separation can no longer be predicted from batch tests.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.002
Threshold uncertainty score0.004

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.006
GPT teacher head0.211
Teacher spread0.205 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations13
Published2017
Admission routes3
Has abstractyes

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