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Record W2644617923 · doi:10.1021/acssuschemeng.7b00615

Cost Reduction and Mechanical Enhancement of Biopolyesters Using an Agricultural Byproduct from Konjac Glucomannan Processing

2017· article· en· W2644617923 on OpenAlexafffund
Zhaoshu Chen, Lin Gan, Peter R. Chang, Changhua Liu, Jin Huang, Shanjun Gao

Bibliographic record

VenueACS Sustainable Chemistry & Engineering · 2017
Typearticle
Languageen
FieldMaterials Science
Topicbiodegradable polymer synthesis and properties
Canadian institutionsAgriculture and Agri-Food Canada
FundersMinistry of Education of the People's Republic of ChinaOffice of Energy Research and DevelopmentChongqing Science and Technology CommissionNational Natural Science Foundation of China
KeywordsUltimate tensile strengthMaterials scienceElongationComposite materialRaw materialCompression moldingDegradation (telecommunications)Polybutylene succinateBiodegradationCompressive strengthIzod impact strength testChemical engineeringChemistryOrganic chemistry

Abstract

fetched live from OpenAlex

Extensive applications of many sustainable biopolyester materials are limited due to their high cost and poor properties. To resolve these problems, we developed a strategy using an agricultural byproduct derived from konjac glucomannan processing, the konjac fly powders (KFPs), to reduce the cost, preserve the biodegradability, and improve the mechanical properties of biopolyesters. The result indicated that the multiple components in KFPs complicate our understanding of the reinforcing mechanism. However, from the tensile and dynamic mechanical behavior, matrix–filler interaction, and fracture morphology of composites, we concluded that the mechanical enhancement of KFPs was selective. By controlling melt mixing and compression molding, the elongation at break and tensile strength of poly(3-hydroxybutyrate- co -4-hydroxybutyrate) (P(3,4)HB) rather than polybutylene succinate (PBS) or polylactide (PLA) could be enhanced by 205% and 111%, respectively, and the cost of composites reduced by 4–22%. Also, the onset degradation temperature of P(3.4)HB at a low KFP loading was about 40 °C higher than neat P(3,4)HB. The enhancing effect of KFPs was mainly attributed to its strong interaction with P(3,4)HB and the homogeneous structure of their composites.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.001

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.025
GPT teacher head0.240
Teacher spread0.214 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations12
Published2017
Admission routes2
Has abstractyes

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