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Record W2737735492

Diffusive Loss of Non-Aqueous Phase Organic Solvents from a Disk Source

2006· dissertation· en· W2737735492 on OpenAlexfundno aff
In-Taek Yoon

Bibliographic record

VenueMacSphere (McMaster University) · 2006
Typedissertation
Languageen
FieldChemical Engineering
TopicChemical and Physical Properties in Aqueous Solutions
Canadian institutionsnot available
FundersMcMaster University
KeywordsAqueous solutionPhase (matter)Aqueous two-phase systemChemistryEnvironmental chemistryEnvironmental scienceChemical engineeringOrganic chemistryEngineering
DOInot available

Abstract

fetched live from OpenAlex

Matrix diffusion from planar fractures was studied both mathematically and through physical model experiments. A conceptual model was developed based on previous work by Parker (1994) and Crank (1956). Mathematical models were developed to simulate diffusion from 2D and 3D instantaneous disk sources and a 3 D continuous disk source. The models were based on analytical solutions previously developed by Carslaw and Jaeger (1959). Analytical solution is not available for the total mass diffused into the porous matrix for a 3D continuous disk source, and it was therefore calculated through the summation of the iso-concentration lines, which were assumed to be a semi-spherical shape. The mathematical simulations indicated that the 2D scenario produces significantly different results from the 3D scenario, the time for mass disappearance is significantly larger for continuous sources than for instantaneous sources, the normalized concentration generally decreased over time for instantaneous sources while it increased over time for continuous sources, diffusion rates decrease significantly over time and space, and the normalized mass loss from the source zone never reaches 1 for continuous sources due to the semi-infinite integral. The simulations also showed that disappearance times increase exponentially with increasing source radii and matrix porosity, and decrease with increasing aqueous-phase NAPL solubilities. The observations from the physical model experiments were very close to the simulated data at z = 0, validating the 3D mathematical models for this elevation. A plot of the observed vs simulated data did not reveal any trends, indicating that the majority of the differences can be attributed to experimental error. The experimental concentrations were below the method detection limit at depths of 3 and 6 cm however, indicating that either the experiments should have been conducted over a longer time period or a more sensitive analytical method should have been employed, to enable model validation at these depths.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Insufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.264
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0360.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.007
GPT teacher head0.198
Teacher spread0.192 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2006
Admission routes1
Has abstractyes

Explore more

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