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Record W2753553828 · doi:10.1021/acs.estlett.7b00355

Tissue Distribution of Substituted Diphenylamine Antioxidants and Benzotriazole Ultraviolet Stabilizers in White Sucker (<i>Catostomus commersonii</i>) from an Urban Creek in Canada

2017· article· en· W2753553828 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.
aboutThe title or abstract carries a Canadian signal from the geographic lexicon.

Bibliographic record

VenueEnvironmental Science & Technology Letters · 2017
Typearticle
Languageen
FieldEnvironmental Science
TopicToxic Organic Pollutants Impact
Canadian institutionsEnvironment and Climate Change Canada
FundersEnvironment and Climate Change Canada
KeywordsDiphenylamineExcretionCatostomusChemistryEnvironmental chemistryBiologyPharmacologyFish <Actinopterygii>BiochemistryFishery

Abstract

fetched live from OpenAlex

Substituted diphenylamine antioxidants (SDPAs) and benzotriazole ultraviolet stabilizers (BZT-UVs) have been detected in aquatic organisms, but little is known about their tissue distribution and elimination in wildlife. This study investigates the distribution of SDPAs and BZT-UVs in blood plasma, bile, liver, and carcass (without gill and internal organs) of white sucker ( Catostomus commersonii ) and evaluates the extent of biliary excretion in fish. Fish were collected from a creek upstream and downstream of an urban area in Ontario, Canada. Downstream fish showed levels of contamination of many target compounds [e.g., 4,4′-bis(α,α-dimethylbenzyl)diphenylamine and monononyl-diphenylamine] higher than those of upstream fish, indicating the input of these contaminants from the urban area. The concentration (wet weight) of target compounds generally decreased in the following order: liver > carcass homogenate ≥ bile > plasma. This indicates that liver is a major tissue for accumulation of these contaminants in fish. Tissue-specific partition coefficients suggest that SDPAs tend to partition from plasma to liver and that the biliary excretion of these contaminants is a relatively minor pathway of elimination. Only monobutyl-diphenylamine was effectively excreted via bile. Our results suggest that future studies should focus on the liver toxicities and biotransformation of these contaminants to improve our understanding of their environmental risks.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Science and technology studies
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Observational · Consensus signal: Observational
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.326
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.004
Scholarly communication0.0000.001
Open science0.0010.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.004
GPT teacher head0.210
Teacher spread0.206 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it