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Record W2759853218 · doi:10.1021/acssuschemeng.7b01556

Fast Drying Boosted Performance Improvement of Low-Temperature Paintable Carbon-Based Perovskite Solar Cell

2017· article· en· W2759853218 on OpenAlexaff
Qianqian Chu, Bin Ding, Yan Li, Lili Gao, Qi Qiu, Cheng-Xin Li, Chang‐Jiu Li, Guan‐Jun Yang, Baizeng Fang

Bibliographic record

VenueACS Sustainable Chemistry & Engineering · 2017
Typearticle
Languageen
FieldEngineering
TopicPerovskite Materials and Applications
Canadian institutionsUniversity of British Columbia
Fundersnot available
KeywordsTrihalideMaterials sciencePerovskite (structure)Carbon fibersEnergy conversion efficiencyGraphiteChemical engineeringPhotovoltaic systemEvaporationSolar cellCarbon blackOpen-circuit voltagePhotovoltaicsNanotechnologyComposite materialOptoelectronicsVoltageChemistryOrganic chemistryElectrical engineeringHalide

Abstract

fetched live from OpenAlex

Low-temperature paintable carbon-based perovskite solar cells have been acknowledged as a promising photovoltaic device. However, the organometal trihalide perovskite film is always degraded by the solvents in the carbon paste, resulting in a fairly low efficiency. Unfortunately, in a conventional drying process, the movements of solvent molecules from a carbon paste to atmosphere are greatly obstructed by the biscale size of carbon black and graphite, which creates an extremely long evaporation path and drying time. To solve the problem, we have developed a simple, highly efficient and scalable method, a gas pump method (GPM), to dry the carbon paste very quickly which demonstrates a 7 times drying rate compared with conventional drying. As a result, the perovskite films covered by the carbon electrode (CE) dried by the GPM keep a uniform and continuous surface morphology, and the champion solar cell reveals a conversion efficiency of 12.30% with the area of 0.1 cm 2 and an open circuit voltage of 1.03 V, which are much higher than those (i.e., 4.73% and 0.81 V, respectively) observed for the PSC without GPM. Furthermore, the long-time stability test shows that the solar cells with the as-prepared CE retain more than 90% of its initial power conversion efficiency after 720 h.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.089
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.002
GPT teacher head0.163
Teacher spread0.161 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations40
Published2017
Admission routes1
Has abstractyes

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